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学者姓名：纪树兰
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Abstract ：
Building up selective mass transfer channels in polymeric membranes is a promising strategy to fabricate effective separation membranes. Herein, a thioether-functionalized hydrazone-linked covalent organic framework, COF-LZU8, pre-modified by Ag ion, was incorporated for constructing aromatic selective channels within a commercial poly (ether-block amide) (Pebax 2533) membrane. The inside nanochannels of resulting membrane were effectively confirmed by measuring the affinity and the selective free volume to toluene via quartz crystal microbalance and low-field nuclear magnetic resonance. Owing to the selective channels, the Ag-COF-LZU8/Pebax membrane presented a considerably enhanced performance for toluene/n-heptane separation comparing with pristine Pebax membranes. The optimized membrane could perform a permeation flux of 293 g/m(2)h and a separation factor of 4.03 for the separation of 50 wt% toluene/n-heptane mixture.
Keyword ：
Aromatic/aliphatic hydrocarbons Aromatic/aliphatic hydrocarbons Covalent organic frameworks (COFs) Covalent organic frameworks (COFs) Hybrid membrane Hybrid membrane Pebax Pebax Pervaporation Pervaporation
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| GB/T 7714 | Zhang, Lilong , Wang, Lin , Wang, Naixin et al. Covalent organic frameworks hybird membrane with optimized mass transport nanochannel for aromatic/aliphatic mixture pervaporation [J]. | JOURNAL OF MEMBRANE SCIENCE , 2020 , 598 . |
| MLA | Zhang, Lilong et al. "Covalent organic frameworks hybird membrane with optimized mass transport nanochannel for aromatic/aliphatic mixture pervaporation" . | JOURNAL OF MEMBRANE SCIENCE 598 (2020) . |
| APA | Zhang, Lilong , Wang, Lin , Wang, Naixin , Guo, Hongxia , Zhang, Wen-Hai , Li, Xiaoting et al. Covalent organic frameworks hybird membrane with optimized mass transport nanochannel for aromatic/aliphatic mixture pervaporation . | JOURNAL OF MEMBRANE SCIENCE , 2020 , 598 . |
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Abstract ：
Recovery of butanol is a potential biofuel production process, which can be achieved through membrane separation technology. In this study, Zeolitic Imidazolate Framework-8 (ZIF-8) modified graphene oxide (ZGO) with polyether block amide (PEBA) was deposited on ceramic tubular substrate to prepare composite membrane for bio-butanol recovery. ZGO laminates can be used to form transport channels for butanol molecules to enhance the permeance. The affinity of laminate to butanol was improved because of the hydrophobic ZIF-8 particles. Therefore, the separation performance of ZGO/PEBA membrane was enhanced. The microstructure and chemical property of the ZGO/PEBA membranes were characterized. Different preparation and operation conditions were also investigated to optimize the separation performance. Moreover, ZGO/PEBA composite membranes were evaluated in model acetone-butanol-ethanol (ABE) solution, which also exhibited high butanol recovery performance. Therefore, this facile strategy may provide a potential application in the commercialized ABE fermentation process.
Keyword ：
Biobutanol recovery Biobutanol recovery PEBA PEBA ZIF-8 ZIF-8 Pervaporation Pervaporation Graphene oxide Graphene oxide
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| GB/T 7714 | Li, Wenhui , Li, Jie , Wang, Naixin et al. Recovery of bio-butanol from aqueous solution with ZIF-8 modified graphene oxide composite membrane [J]. | JOURNAL OF MEMBRANE SCIENCE , 2020 , 598 . |
| MLA | Li, Wenhui et al. "Recovery of bio-butanol from aqueous solution with ZIF-8 modified graphene oxide composite membrane" . | JOURNAL OF MEMBRANE SCIENCE 598 (2020) . |
| APA | Li, Wenhui , Li, Jie , Wang, Naixin , Li, Xiaoting , Zhang, Yifan , Ye, Qing et al. Recovery of bio-butanol from aqueous solution with ZIF-8 modified graphene oxide composite membrane . | JOURNAL OF MEMBRANE SCIENCE , 2020 , 598 . |
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| GB/T 7714 | Wang, Naixin , Li, Qian , Li, Xiaoting et al. Vacuum -assisted assembly of iron cage intercalated layered double hydroxide composite membrane for water purification [J]. | JOURNAL OF MEMBRANE SCIENCE , 2020 , 603 . |
| MLA | Wang, Naixin et al. "Vacuum -assisted assembly of iron cage intercalated layered double hydroxide composite membrane for water purification" . | JOURNAL OF MEMBRANE SCIENCE 603 (2020) . |
| APA | Wang, Naixin , Li, Qian , Li, Xiaoting , Zhang, Wenhai , Ji, Shulan , An, Quan-Fu . Vacuum -assisted assembly of iron cage intercalated layered double hydroxide composite membrane for water purification . | JOURNAL OF MEMBRANE SCIENCE , 2020 , 603 . |
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Abstract ：
A defect-free, robust and selective barrier is essential for manufacturing membranes with targeted high permeability and selectivity. Here we report a new route to engineering a separation composite membrane by confining both channels in nanoscale metal organic frameworks (MOFs) and charges in a polyelectrolyte in the inner space of a porous supportviaa counter-diffusion method. A simple thermal annealing treatment of the interface between the MOF, polymer and support favorably reduced voids inside this nano-confinement environment. As this composite membrane combines both the support and barrier as one, it minimizes mass transfer resistance of water molecules. In a separation test, it readily achieved the state-of-the-art permeance. This simple chemical approach to upgrade membrane structures will offer wide opportunities in separation devices.
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| GB/T 7714 | Li, Xiaoting , Wang, Naixin , Bao, Xinmin et al. Nano-confinement-inspired metal organic framework/polymer composite separation membranes [J]. | JOURNAL OF MATERIALS CHEMISTRY A , 2020 , 8 (33) : 17212-17218 . |
| MLA | Li, Xiaoting et al. "Nano-confinement-inspired metal organic framework/polymer composite separation membranes" . | JOURNAL OF MATERIALS CHEMISTRY A 8 . 33 (2020) : 17212-17218 . |
| APA | Li, Xiaoting , Wang, Naixin , Bao, Xinmin , Li, Qian , Li, Jie , Xie, Ya-Bo et al. Nano-confinement-inspired metal organic framework/polymer composite separation membranes . | JOURNAL OF MATERIALS CHEMISTRY A , 2020 , 8 (33) , 17212-17218 . |
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Abstract ：
Organic solvent nanofiltration (OSN) is an emerging membrane-based technology for molecular separation. The design and fabrication of membranes with unique structures are important to obtain high performance. Herein, ZIF-8 nanoparticles are grown in situ on the surface of graphene oxide (GO) nanosheets and then assembled on a tubular ceramic substrate through a vacuum-assisted assembly method. ZIF-8 anchored on the GO nanosheets is evolved into ZnS polyhedra with a hollow structure through in situ sulfurization. The formed ZnS@GO membrane is composed of a layered structure of GO with the interlayer intercalated by ZnS hollow polyhedra and demonstrates high permeance for organic solvents. Compared to that of the ZIF-8@GO membrane, the permeance of the ZnS@GO membrane is enhanced by 4.4-fold when separating dyes from methanol, indicating their promising potential in the application of organic solvent nanofiltration.
Keyword ：
graphene oxide graphene oxide ZIF-8 derivatives ZIF-8 derivatives organic solvent nanofiltration organic solvent nanofiltration high permeance high permeance in situ sulfurization in situ sulfurization
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| GB/T 7714 | Wang, Naixin , Sun, Hao , Yang, Hengyu et al. Hollow Polyhedron-Modified Graphene Oxide Membranes for Organic Solvent Nanofiltration with Enhanced Permeance [J]. | ACS APPLIED NANO MATERIALS , 2020 , 3 (6) : 5874-5880 . |
| MLA | Wang, Naixin et al. "Hollow Polyhedron-Modified Graphene Oxide Membranes for Organic Solvent Nanofiltration with Enhanced Permeance" . | ACS APPLIED NANO MATERIALS 3 . 6 (2020) : 5874-5880 . |
| APA | Wang, Naixin , Sun, Hao , Yang, Hengyu , Li, Xiaoting , Ji, Shulan , An, Quan-Fu . Hollow Polyhedron-Modified Graphene Oxide Membranes for Organic Solvent Nanofiltration with Enhanced Permeance . | ACS APPLIED NANO MATERIALS , 2020 , 3 (6) , 5874-5880 . |
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Abstract ：
Organic solvent nanofiltration (OSN) is emerging as an efficient and emerging approach for separation and purification of solute from organic solvents, which however were severely underdeveloped because of the low permeance of membranes. Herein, a novel mixed matrix membrane (MMM) was developed by incorporation of modified mesoporous silica nanoparticle (MSN) into commercially-available polydimethylsiloxane (PDMS) matrix for removal of trace impurities, such as Evans blue or vitamin B12, from different organic solvents. Notably, because of the designed nanoscale spaces originated from MSN, the permeance of the optimized MMM reached up to 31.2 L m(-2).h(-1).MPa-1, around 17-fold enhancement compared with that of pristine PDMS membrane. Low-field nuclear magnetic resonance was employed to trace the solvent state in the MMM. The MMM exhibited high MeOH absorption capability but low-swelling attribute, certificating the high permeance and long-term stability of the MMM. The MMM was stably tested in MeOH solution for more than 80 h, indicating the great promise for future practical OSN applications.
Keyword ：
Nanohybrid Nanohybrid Low-field nuclear magnetic resonance Low-field nuclear magnetic resonance Organic solvent nanofiltration Organic solvent nanofiltration Mesoporous silica nanoparticles Mesoporous silica nanoparticles Polydimethylsiloxane Polydimethylsiloxane
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| GB/T 7714 | Li, Chong , Li, Jie , Zhang, Wen-Hai et al. Enhanced permeance for PDMS organic solvent nanofiltration membranes using modified mesoporous silica nanoparticles [J]. | JOURNAL OF MEMBRANE SCIENCE , 2020 , 612 . |
| MLA | Li, Chong et al. "Enhanced permeance for PDMS organic solvent nanofiltration membranes using modified mesoporous silica nanoparticles" . | JOURNAL OF MEMBRANE SCIENCE 612 (2020) . |
| APA | Li, Chong , Li, Jie , Zhang, Wen-Hai , Wang, Naixin , Ji, Shulan , An, Quan-Fu . Enhanced permeance for PDMS organic solvent nanofiltration membranes using modified mesoporous silica nanoparticles . | JOURNAL OF MEMBRANE SCIENCE , 2020 , 612 . |
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Abstract ：
一种制备Fe‑cage插层层状双金属氢氧化物纳滤膜的方法，属于纳滤膜分离领域。其步骤包括：对多孔基膜进行预处理，使其荷负电，去除表面杂质，并对其进行水解；将金属盐、尿素溶解于乙二醇中，搅拌均匀后将其置于高压反应釜中反应，以此制备LDH纳米片；采用金属‑有机自组装法制备Fe‑cage；通过Fe‑cage调节LDH纳米片之间形成的纳米通道的结构和化学性质，采用真空辅助法在多孔基膜上沉积LDH/Fe‑cage，形成薄膜分离层；本发明有效提高纳滤膜的分离性及稳定性。该方法制备简单，成膜快，还可用于制备具有不同嵌入分子的LDH膜以用于其它应用。
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| GB/T 7714 | 王乃鑫 , 李倩 , 韩旺 et al. 一种制备Fe-cage插层层状双金属氢氧化物纳滤膜的方法 : CN201911029909.9[P]. | 2019-10-26 . |
| MLA | 王乃鑫 et al. "一种制备Fe-cage插层层状双金属氢氧化物纳滤膜的方法" : CN201911029909.9. | 2019-10-26 . |
| APA | 王乃鑫 , 李倩 , 韩旺 , 安全福 , 纪树兰 . 一种制备Fe-cage插层层状双金属氢氧化物纳滤膜的方法 : CN201911029909.9. | 2019-10-26 . |
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Abstract ：
一种过渡金属离子改性共价有机骨架/聚合物杂化膜、制备及应用，属于膜分离领域。其步骤包括：以COFs中极性基团作为络合点，将过渡金属离子引入到COFs结构中，对其进行改性，得到过渡金属离子改性的COFs(M‑COFs)；采用湿法研磨及超声搅拌的方式制备分散均匀的M‑COFs/聚合物成膜液；通过简单浸渍提拉法在无机多孔膜表面复合M‑COFs/聚合物，形成薄膜分离层。本发明利用过渡金属离子与COFs中极性基团的作用，将过渡金属离子引入到COFs中以提高COFs与芳烃的亲和性，继而进一步增强所制备的杂化膜对芳烃/烷烃体系的选择性。
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| GB/T 7714 | 安全福 , 张丽龙 , 王乃鑫 et al. 一种过渡金属离子改性共价有机骨架/聚合物杂化膜、制备及应用 : CN201911048814.1[P]. | 2019-10-31 . |
| MLA | 安全福 et al. "一种过渡金属离子改性共价有机骨架/聚合物杂化膜、制备及应用" : CN201911048814.1. | 2019-10-31 . |
| APA | 安全福 , 张丽龙 , 王乃鑫 , 汪林 , 张文海 , 纪树兰 . 一种过渡金属离子改性共价有机骨架/聚合物杂化膜、制备及应用 : CN201911048814.1. | 2019-10-31 . |
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Abstract ：
NaA membranes are recognized as one of the most promising materials for fabrication of high-performance pervaporation membrane for dehydration, which has been widely employed in dehydration industry. However, the chemical structure breakage of NaA in acidic conditions severely hampered the application of NaA membrane in purification of biomass fermentation. In order to overcome this bottleneck, we proposed construction of a protective acid-resistant skin on the 3D surface of NaA tube. The protective layer was prepared by self-assembly of sodium alginate (SA) and CaCl2, which formed the 'egg-box' network via crosslinking SA with Ca2+. The effect of cross-linking, SA concentration, layer numbers and operation pH on the membrane performance was investigated. When applied for pervaporation at acidic feed, the protective skin was partly broken, but it can be re-crosslinked again by simple ionic exchange to form a solid acid-resistant skin. After the re-crosslinking treatment, the performance of membrane can be recovered (the water content in the permeate and the flux were 99.6 wt% and 860 g/(m(2)h), respectively) with operation condition at pH = 2. Notably, the membrane can be continuously operated in acid feed for 100 h and showed no obvious performance degradation.
Keyword ：
Acid-resistant Acid-resistant NaA NaA Pervaporation Pervaporation Re-crosslinking Re-crosslinking
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| GB/T 7714 | Li, Jie , Li, Chong , Li, Xiaoqing et al. 3D re-crosslinking of an acid-resistant layer on NaA tubular membrane for application in acidic feed [J]. | JOURNAL OF MEMBRANE SCIENCE , 2019 , 589 . |
| MLA | Li, Jie et al. "3D re-crosslinking of an acid-resistant layer on NaA tubular membrane for application in acidic feed" . | JOURNAL OF MEMBRANE SCIENCE 589 (2019) . |
| APA | Li, Jie , Li, Chong , Li, Xiaoqing , Wang, Naixin , Ji, Shulan , An, Quan-Fu . 3D re-crosslinking of an acid-resistant layer on NaA tubular membrane for application in acidic feed . | JOURNAL OF MEMBRANE SCIENCE , 2019 , 589 . |
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Abstract ：
一种制备Fe‑cage插层层状双金属氢氧化物纳滤膜的方法，属于纳滤膜分离领域。其步骤包括：对多孔基膜进行预处理，使其荷负电，去除表面杂质，并对其进行水解；将金属盐、尿素溶解于乙二醇中，搅拌均匀后将其置于高压反应釜中反应，以此制备LDH纳米片；采用金属‑有机自组装法制备Fe‑cage；通过Fe‑cage调节LDH纳米片之间形成的纳米通道的结构和化学性质，采用真空辅助法在多孔基膜上沉积LDH/Fe‑cage，形成薄膜分离层；本发明有效提高纳滤膜的分离性及稳定性。该方法制备简单，成膜快，还可用于制备具有不同嵌入分子的LDH膜以用于其它应用。
Cite：
Copy from the list or Export to your reference management。
| GB/T 7714 | 王乃鑫 , 李倩 , 韩旺 et al. 一种制备Fe-cage插层层状双金属氢氧化物纳滤膜的方法 : CN201911029909.9[P]. | 2019-10-26 . |
| MLA | 王乃鑫 et al. "一种制备Fe-cage插层层状双金属氢氧化物纳滤膜的方法" : CN201911029909.9. | 2019-10-26 . |
| APA | 王乃鑫 , 李倩 , 韩旺 , 安全福 , 纪树兰 . 一种制备Fe-cage插层层状双金属氢氧化物纳滤膜的方法 : CN201911029909.9. | 2019-10-26 . |
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