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摘要:
A total of 15 light-duty diesel vehicles (LDDVs) were tested with the goal of understanding the emission factors of real-world vehicles by conducting on-board emission measurements. The emission characteristics of hydrocarbons (HC) and nitrogen oxides (NOx) at different speeds, chemical species profiles and ozone formation potential (OFP) of volatile organic compounds (VOCs) emitted from diesel vehicles with different emission standards were analyzed. The results demonstrated that emission reductions of HC and NO,, had been achieved as the control technology became more rigorous from Stage I to Stage IV. It was also found that the HC and NO emissions and percentage of O-2 dropped with the increase of speed, while the percentage of CO2 increased. The abundance of alkanes was significantly higher in diesel vehicle emissions, approximately accounting for 41.1%-45.2%, followed by aromatics and alkenes. The most abundant species were propene, ethane, n-decane, n-undecane, and n-dodecane. The maximum incremental reactivity (MIR) method was adopted to evaluate the contributions of individual VOCs to OFP. The results indicated that the largest contributors to O-3 production were alkenes and aromatics, which accounted for 87.7%-91.5%. Propene, ethene, 1,2,4-trimethylbenzene, 1-butene, and 1,2,3-trimethylbenzene were the top five VOC species based on their OFP, and accounted for 54.0%-64.8% of the total OFP. The threshold dilution factor was applied to analyze the possibility of VOC stench pollution. The majority of stench components emitted from vehicle exhaust were aromatics, especially p-diethylbenzene, propylbenzene, m-ethyltoluene, and p-ethyltoluene. (C) 2016 The Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences. Published by Elsevier B.V.
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通讯作者信息:
来源 :
JOURNAL OF ENVIRONMENTAL SCIENCES
ISSN: 1001-0742
年份: 2016
卷: 46
页码: 28-37
6 . 9 0 0
JCR@2022
ESI学科: ENVIRONMENT/ECOLOGY;
ESI高被引阀值:145
中科院分区:3