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作者:

Zhang, Wenxiang (Zhang, Wenxiang.) | Ding, Luhui (Ding, Luhui.) | Zhang, Zhien (Zhang, Zhien.) | Wei, Jia (Wei, Jia.) (学者:魏佳) | Jaffrin, Michel Y. (Jaffrin, Michel Y..) | Huang, Guohe (Huang, Guohe.)

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EI Scopus SCIE

摘要:

Micellar enhanced ultrafiltration is a promising technology for removing trace amounts of organic pollutants in wastewater, but membrane fouling caused by Gemini micelles is a significant problem restricting its industrial application. In this study, a flat sheet ultrafiltration membrane with four types of Gemini surfactant systems and various feed concentrations was used to treat phenol wastewater, while the flux behavior and fouling mechanism were investigated. The optimal permeate flux of phenol decreased in the sequence as follows: CG(12) > CG(16) > CG(12) - Brij35 > CG(16) - Brij35. In order to study the rate of membrane fouling, a developed liner regression method was utilized to help determine the threshold flux, as well the degree of concentration polarization and membrane fouling. Furthermore, limiting flux was investigated to avoid extensive cake layer formation. Threshold flux and limiting flux strongly depended on the feed concentration and the type of micelles. The threshold flux reduced gradually with feed concentration, due to the increased fouling rate and presence of irreversible fouling. Owing to the effect of charge density and hydrophobicity of micelles, CG(12) exhibited the highest threshold flux and limiting flux. Flux-TMP relation was divided into three regions for analyzing the corresponding changes of permeate flux, filtration resistance and conceptual particle deposition model. Besides, fouling mechanism of MEUF was discussed. This study provides a guideline for analyzing membrane fouling and seeking an optimum operation strategy for controlling fouling in membrane water treatment. (C) 2015 Elsevier Ltd. All rights reserved.

关键词:

Micellar enhanced ultrafiltration Fouling control Threshold flux Membrane fouling Limiting flux

作者机构:

  • [ 1 ] [Zhang, Wenxiang]Univ Technol Compiegne, EA TIMR 4297, F-60205 Compiegne, France
  • [ 2 ] [Ding, Luhui]Univ Technol Compiegne, EA TIMR 4297, F-60205 Compiegne, France
  • [ 3 ] [Zhang, Wenxiang]North China Elect Power Univ, Resources & Environm Res Acad, MOE Key Lab Reg Energy & Environm Syst Optimizat, Beijing 102206, Peoples R China
  • [ 4 ] [Huang, Guohe]North China Elect Power Univ, Resources & Environm Res Acad, MOE Key Lab Reg Energy & Environm Syst Optimizat, Beijing 102206, Peoples R China
  • [ 5 ] [Zhang, Zhien]Chongqing Univ, Coll Power Engn, Chongqing 400044, Peoples R China
  • [ 6 ] [Wei, Jia]Beijing Univ Technol, Key Lab Beijing Water Qual Sci & Water Environm R, Beijing 100124, Peoples R China
  • [ 7 ] [Jaffrin, Michel Y.]Univ Technol Compiegne, UMR7338, F-60205 Compiegne, France

通讯作者信息:

  • [Zhang, Wenxiang]Univ Technol Compiegne, EA TIMR 4297, F-60205 Compiegne, France

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来源 :

JOURNAL OF CLEANER PRODUCTION

ISSN: 0959-6526

年份: 2016

卷: 112

页码: 1241-1251

1 1 . 1 0 0

JCR@2022

ESI学科: ENGINEERING;

ESI高被引阀值:166

中科院分区:2

被引次数:

WoS核心集被引频次: 22

SCOPUS被引频次: 30

ESI高被引论文在榜: 0 展开所有

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