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作者:

Wang, Litao (Wang, Litao.) | Wei, Zhe (Wei, Zhe.) | Wei, Wei (Wei, Wei.) | Fu, Joshua S. (Fu, Joshua S..) | Meng, Chenchen (Meng, Chenchen.) | Ma, Simeng (Ma, Simeng.)

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EI Scopus SCIE

摘要:

Hebei has been recognized as one of the most polluted provinces in China, characterized by extremely high concentrations of fine particulate matter (PM2.5) in many of its cities, especially those located in the southern area of the province and highly potentially northward transported to Beijing. Source apportionment of PM2.5 is the basis and prerequisite of an effective control strategy. In this study, the Mesoscale Modeling System Generation 5 (MM5) and the Models-3/Community Multiscale Air Quality (CMAQ) modeling system are applied to East Asia and North China at 36- and 12-km horizontal grid resolutions, and the source apportionment of PM2.5 in the three top polluted cities in Hebei, i.e., Shijiazhuang, Xingtai, and Handan, is performed using the Brute-Force method. It is concluded that the regional source contributions to PM2.5 are 27.9% in Shijiazhuang, 46.6% in Xingtai, and 40.4% in Handan. The major local contributors are industrial, domestic and agricultural sources in all the three cities with the contributions of 39.8%, 15.8%, and 10.6% in Shijiazhuang, 30.5%, 13.6%, and 6.9% in Xingtai, 35.9%, 13.5%, and 6.2% in Handan, respectively. As to the secondary aerosols of sulfate (SO42-), nitrate (NO3-), and ammonium (NH4+) in PM2.5, which are important chemical species in PM2.5 (about 30-40% in PM2.5) and cannot be further apportioned by receptor models, the regional source contributions to the total concentrations of SO42-, NO3-, and NH4+ are 40.9%, 62.0%, and 59.1% in Shijiazhuang, Xingtai, and Handan, respectively. The local industrial, domestic and agricultural contributions to those are 23.7%, 6.6%, and 29.8% in total in Shijiazhuang, 17.5%, 5.0%, and 17.7% in Xingtai, and 20.6%, 4.8%, and 17.8% in Handan, respectively. The regional joint controls of air pollution are more important in Xingtai and Handan than in Shijiazhuang, and the emission controls of agricultural sources need to be further considered in the future policy. (C) 2015 Elsevier Ltd. All rights reserved.

关键词:

PM2.5 Source apportionment Hebei Secondary aerosol MM5-CMAQ

作者机构:

  • [ 1 ] [Wang, Litao]Hebei Univ Engn, Sch City Construct, Dept Environm Engn, Handan 056038, Hebei, Peoples R China
  • [ 2 ] [Wei, Zhe]Hebei Univ Engn, Sch City Construct, Dept Environm Engn, Handan 056038, Hebei, Peoples R China
  • [ 3 ] [Meng, Chenchen]Hebei Univ Engn, Sch City Construct, Dept Environm Engn, Handan 056038, Hebei, Peoples R China
  • [ 4 ] [Ma, Simeng]Hebei Univ Engn, Sch City Construct, Dept Environm Engn, Handan 056038, Hebei, Peoples R China
  • [ 5 ] [Wang, Litao]Univ Tennessee, Dept Civil & Environm Engn, Knoxville, TN 37996 USA
  • [ 6 ] [Fu, Joshua S.]Univ Tennessee, Dept Civil & Environm Engn, Knoxville, TN 37996 USA
  • [ 7 ] [Wei, Wei]Beijing Univ Technol, Dept Environm Sci, Beijing 100124, Peoples R China

通讯作者信息:

  • [Wang, Litao]Hebei Univ Engn, Sch City Construct, Dept Environm Engn, Handan 056038, Hebei, Peoples R China

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来源 :

ATMOSPHERIC ENVIRONMENT

ISSN: 1352-2310

年份: 2015

卷: 122

页码: 723-736

5 . 0 0 0

JCR@2022

ESI学科: GEOSCIENCES;

ESI高被引阀值:204

JCR分区:1

中科院分区:2

被引次数:

WoS核心集被引频次: 101

SCOPUS被引频次: 114

ESI高被引论文在榜: 0 展开所有

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