The　design　principles　for　naturally　occurring　biological　materials　have　inspired　us　to　develop　next-generation　engineering　materials　with　remarkable　performance.　Nacre,　commonly　referred　to　as　nature＇s　armor,　is　renowned　for　its　unusual　combination　of　strength　and　toughness.　Nature＇s　wisdom　in　nacre　resides　in　its　elaborate　structural　design　and　the　judicious　placement　of　a　unique　organic　biopolymer　with　intelligent　deformation　features.　However,　up　to　now,　it　is　still　a　challenge　to　transcribe　the　biopolymer＇s　deformation　attributes　into　a　stronger　substitute　in　the　design　of　new　materials.　In　this　study,　we　propose　a　new　design　strategy　that　employs　shape　memory　alloy　to　transcribe　the　＂J-curve＇＇　mechanical　response　and　uniform　molecular/atomic　level　deformation　of　the　organic　biopolymer　in　the　design　of　high-performance　hybrid　materials.　This　design　strategy　is　verified　in　a　TiNi-Ti3Sn　model　material　system.　The　model　material　demonstrates　an　exceptional　combination　of　mechanical　properties　that　are　superior　to　other　high-performance　metal-based　lamellar　composites　known　to　date.　Our　design　strategy　creates　new　opportunities　for　the　development　of　high-performance　bio-inspired　materials.