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作者:

Ma Xuyi (Ma Xuyi.) | Zhang Xin (Zhang Xin.) | Lu Qingmei (Lu Qingmei.) | Zhang Jiuxing (Zhang Jiuxing.)

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EI Scopus SCIE PKU CSCD

摘要:

Bismuth and Tellurium nanoparticles were prepared by evaporation-condensation method in argon atmosphere, and n-type Bi2Te3 fine-grained thermoelectric bulk materials were fabricated by spark plasma sintering (SPS) at different temperatures from 663 to 723 K using mechanically alloyed (MA) powders. The phase compositions of powder and bulk samples were characterized by X-ray diffraction (XRD). The sizes and microscopic structures of nanoparticles and fractured cross section of the bulk samples were observed by transmission electron microscopy (TEM) and scanning electron microscopy (SEM), respectively. The thermoelectric transport properties were measured at 323 similar to 473 K. The results show that electrical transport properties are almost unchanged but thermal conductivity is reduced significantly from 1.93 W/m.K to 1.29 W/m.K at 423 K for the fine-grained bulks prepared by nanoparticles comparing with coarse-grained materials. The maximum ZT value after SPS at 693 K reaches 0.68 at 423 K.

关键词:

thermal conductivity thermoelectric properties n-type bulk Bi2Te3 evaporation-condensation spark plasma sintering

作者机构:

  • [ 1 ] [Ma Xuyi]Beijing Univ Technol, Key Lab Adv Funct Mat, Minist Educ, Beijing 100124, Peoples R China
  • [ 2 ] [Zhang Xin]Beijing Univ Technol, Key Lab Adv Funct Mat, Minist Educ, Beijing 100124, Peoples R China
  • [ 3 ] [Lu Qingmei]Beijing Univ Technol, Key Lab Adv Funct Mat, Minist Educ, Beijing 100124, Peoples R China
  • [ 4 ] [Zhang Jiuxing]Beijing Univ Technol, Key Lab Adv Funct Mat, Minist Educ, Beijing 100124, Peoples R China

通讯作者信息:

  • [Ma Xuyi]Beijing Univ Technol, Key Lab Adv Funct Mat, Minist Educ, Beijing 100124, Peoples R China

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来源 :

RARE METAL MATERIALS AND ENGINEERING

ISSN: 1002-185X

年份: 2012

期: 6

卷: 41

页码: 1097-1100

0 . 7 0 0

JCR@2022

ESI学科: MATERIALS SCIENCE;

JCR分区:4

中科院分区:4

被引次数:

WoS核心集被引频次: 5

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