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作者:

Liang, Wen-Jun (Liang, Wen-Jun.) (学者:梁文俊) | Fang, Hong-Ping (Fang, Hong-Ping.) | Li, Jian (Li, Jian.) | Zheng, Feng (Zheng, Feng.) | Li, Jing-Xin (Li, Jing-Xin.) | Jin, Yu-Quan (Jin, Yu-Quan.)

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摘要:

Destruction of hydrogen sulfide using dielectric barrier discharge plasma in a coaxial cylindrical reactor was carried out at atmospheric pressure and room temperature. Three types of DBD reactor were compared in terms of specific energy density (SED), equivalent capacitances of the gap (Cg) and the dielectric barrier (Cd), energy yield (EY), and H2S decomposition. In addition, byproducts during the decomposition of H2S and destruction mechanism were also investigated. SED for all the reactors depended almost linearly on the voltage. In general, Cg decreased with increasing voltage and with the existence of pellet material, while Cd displayed the opposite trend. The removal efficiency of H2S increased substantially with increasing AC frequency and applied voltage. Longer gas residence times also contributed to higher H2S removal efficiency. The choice of pellet material was an important factor influencing the H2S removal. The reactor filled with ceramic Raschig rings had the best H2S removal performance, with an EY of 7.30 g/kWh. The likely main products in the outlet effluent were H2O, SO2, and SO3. (C) 2011 Elsevier B.V. All rights reserved.

关键词:

Dielectric barrier discharge Hydrogen sulfide Lissajous diagram Non-thermal plasma Specific energy density

作者机构:

  • [ 1 ] [Liang, Wen-Jun]Beijing Univ Technol, Coll Environm & Energy Engn, Beijing 100124, Peoples R China
  • [ 2 ] [Fang, Hong-Ping]Beijing Univ Technol, Coll Environm & Energy Engn, Beijing 100124, Peoples R China
  • [ 3 ] [Li, Jian]Beijing Univ Technol, Coll Environm & Energy Engn, Beijing 100124, Peoples R China
  • [ 4 ] [Zheng, Feng]Beijing Univ Technol, Coll Environm & Energy Engn, Beijing 100124, Peoples R China
  • [ 5 ] [Li, Jing-Xin]Beijing Univ Technol, Coll Environm & Energy Engn, Beijing 100124, Peoples R China
  • [ 6 ] [Jin, Yu-Quan]Beijing Univ Technol, Coll Environm & Energy Engn, Beijing 100124, Peoples R China

通讯作者信息:

  • 梁文俊

    [Liang, Wen-Jun]Beijing Univ Technol, Coll Environm & Energy Engn, 100 Ping Le Yuan, Beijing 100124, Peoples R China

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来源 :

JOURNAL OF ELECTROSTATICS

ISSN: 0304-3886

年份: 2011

期: 3

卷: 69

页码: 206-213

1 . 8 0 0

JCR@2022

ESI学科: ENGINEERING;

ESI高被引阀值:155

JCR分区:2

中科院分区:3

被引次数:

WoS核心集被引频次: 52

SCOPUS被引频次: 57

ESI高被引论文在榜: 0 展开所有

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