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Author:

Song, Junhua (Song, Junhua.) | Wang, Kuan (Wang, Kuan.) | Zheng, Jianming (Zheng, Jianming.) | Engelhard, Mark H. (Engelhard, Mark H..) | Xiao, Biwei (Xiao, Biwei.) | Hu, Enyuan (Hu, Enyuan.) | Zhu, Zihua (Zhu, Zihua.) | Wang, Chongmin (Wang, Chongmin.) | Sui, Manling (Sui, Manling.) (Scholars:隋曼龄) | Lin, Yuehe (Lin, Yuehe.) | Reed, David (Reed, David.) | Sprenkle, Vincent L. (Sprenkle, Vincent L..) | Yan, Pengfei (Yan, Pengfei.) (Scholars:闫鹏飞) | Li, Xiaolin (Li, Xiaolin.)

Indexed by:

EI Scopus SCIE

Abstract:

O3-layered metal oxides are promising cathode materials for high-energy Na-ion batteries (SIBs); however, they suffer from fast capacity fade. Here, we develop a high-performance O3-Na-Ni0.68Mn0.22Co0.10O2 cathode for SIBs toward practical applications by suppressing the formation of a rock salt layer at the cathode surface with an advanced electrolyte. The cathode can deliver a high specific capacity of similar to 196 mAh g(-1) and demonstrates >80% capacity retention over 1000 cycles. NaNi0.68Mn0.22Co0.10O2-hard carbon full-cells with practical loading (>2.5 mAh cm-2) and lean electrolyte (similar to 40 mu L) demonstrate similar to 82% capacity retention after 450 cycles. A 60 mAh single-layer pouch cell has also been fabricated and demonstrated stable performance. This work represents a significant leap in SIB development and brings new insights to the development of advanced layered metal oxide cathodes for alkaline-ion batteries.

Keyword:

Author Community:

  • [ 1 ] [Song, Junhua]Pacific Northwest Natl Lab, Richland, WA 99352 USA
  • [ 2 ] [Zheng, Jianming]Pacific Northwest Natl Lab, Richland, WA 99352 USA
  • [ 3 ] [Engelhard, Mark H.]Pacific Northwest Natl Lab, Richland, WA 99352 USA
  • [ 4 ] [Xiao, Biwei]Pacific Northwest Natl Lab, Richland, WA 99352 USA
  • [ 5 ] [Zhu, Zihua]Pacific Northwest Natl Lab, Richland, WA 99352 USA
  • [ 6 ] [Wang, Chongmin]Pacific Northwest Natl Lab, Richland, WA 99352 USA
  • [ 7 ] [Reed, David]Pacific Northwest Natl Lab, Richland, WA 99352 USA
  • [ 8 ] [Sprenkle, Vincent L.]Pacific Northwest Natl Lab, Richland, WA 99352 USA
  • [ 9 ] [Li, Xiaolin]Pacific Northwest Natl Lab, Richland, WA 99352 USA
  • [ 10 ] [Song, Junhua]Washington State Univ, Sch Mech & Mat Engn, Pullman, WA 99164 USA
  • [ 11 ] [Lin, Yuehe]Washington State Univ, Sch Mech & Mat Engn, Pullman, WA 99164 USA
  • [ 12 ] [Wang, Kuan]Beijing Univ Technol, Inst Microstruct & Properties Adv Mat, Beijing Key Lab Microstruct & Properties Solids, Beijing 100124, Peoples R China
  • [ 13 ] [Sui, Manling]Beijing Univ Technol, Inst Microstruct & Properties Adv Mat, Beijing Key Lab Microstruct & Properties Solids, Beijing 100124, Peoples R China
  • [ 14 ] [Yan, Pengfei]Beijing Univ Technol, Inst Microstruct & Properties Adv Mat, Beijing Key Lab Microstruct & Properties Solids, Beijing 100124, Peoples R China
  • [ 15 ] [Hu, Enyuan]Brookhaven Natl Lab, Chem Div, Upton, NY 11973 USA

Reprint Author's Address:

  • 闫鹏飞

    [Zheng, Jianming]Pacific Northwest Natl Lab, Richland, WA 99352 USA;;[Li, Xiaolin]Pacific Northwest Natl Lab, Richland, WA 99352 USA;;[Lin, Yuehe]Washington State Univ, Sch Mech & Mat Engn, Pullman, WA 99164 USA;;[Yan, Pengfei]Beijing Univ Technol, Inst Microstruct & Properties Adv Mat, Beijing Key Lab Microstruct & Properties Solids, Beijing 100124, Peoples R China

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Source :

ACS ENERGY LETTERS

ISSN: 2380-8195

Year: 2020

Issue: 6

Volume: 5

Page: 1718-1725

2 2 . 0 0 0

JCR@2022

Cited Count:

WoS CC Cited Count: 91

SCOPUS Cited Count: 90

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 4

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