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作者:

Yao, Shiyin (Yao, Shiyin.) | Wei, Wei (Wei, Wei.) | Cheng, Shuiyuan (Cheng, Shuiyuan.) (学者:程水源) | Niu, Yuan (Niu, Yuan.) | Guan, Panbo (Guan, Panbo.)

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EI Scopus SCIE

摘要:

The air quality of Handan, a typical industrial city in China, has been significantly improved through atmospheric pollution control, except for ozone (O-3) pollution. We found that, in summer, emissions of anthropogenic volatile organic compounds (VOCs) and NOx decreased yearly in Handan, but the O-3 concentration significantly declined yearly during 2013-2015, whereas it experienced worsening O-3 pollution after 2015. Therefore, we used the Weather Research and Forecasting Community Multiscale Air Quality (WRF-CMAQ) modeling system to simulate the influence of the meteorological conditions and emission changes in Handan during the typical period (June) of O-3 pollution in 2013-2018. For benchmarked June 2013, the results showed that the reduction of the O-3 concentration in June of 2014-2016 was mainly caused by emission reduction, while in June of 2017-2018, the combined effect of changes in emissions and meteorological conditions led to aggravated O-3 pollution. Sensitivity analysis indicated that combined VOCs and NOx emission controls would effectively reduce incremental O-3 formation when the abatement ratio of VOCs/NOx should be no less than 0.84, and we found that VOCs reduction would continusouly bring about O-3 decreases under various NOx reductions, but its positive sensitivity to O-3 would become smaller with NOx reduction. However, the positive influence of NOx reduction on O-3 would happen until NOx reduction exceeding 45-60%. The findings will be helpful in formulating emission control strategies for coping with O-3 pollution in an industrial city.

关键词:

surface ozone quantitative assessment WRF-CMAQ model system control strategy

作者机构:

  • [ 1 ] [Yao, Shiyin]Beijing Univ Technol, Key Lab Beijing Reg Air Pollut Control, Beijing 100124, Peoples R China
  • [ 2 ] [Wei, Wei]Beijing Univ Technol, Key Lab Beijing Reg Air Pollut Control, Beijing 100124, Peoples R China
  • [ 3 ] [Cheng, Shuiyuan]Beijing Univ Technol, Key Lab Beijing Reg Air Pollut Control, Beijing 100124, Peoples R China
  • [ 4 ] [Niu, Yuan]Beijing Univ Technol, Key Lab Beijing Reg Air Pollut Control, Beijing 100124, Peoples R China
  • [ 5 ] [Guan, Panbo]Beijing Univ Technol, Key Lab Beijing Reg Air Pollut Control, Beijing 100124, Peoples R China

通讯作者信息:

  • [Wei, Wei]Beijing Univ Technol, Key Lab Beijing Reg Air Pollut Control, Beijing 100124, Peoples R China

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来源 :

ATMOSPHERE

年份: 2021

期: 5

卷: 12

2 . 9 0 0

JCR@2022

ESI学科: GEOSCIENCES;

ESI高被引阀值:64

JCR分区:3

被引次数:

WoS核心集被引频次: 10

SCOPUS被引频次: 11

ESI高被引论文在榜: 0 展开所有

万方被引频次:

中文被引频次:

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