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作者:

Li, Shuaishuai (Li, Shuaishuai.) | Zeng, Wei (Zeng, Wei.) (学者:曾薇) | Ren, Ziyan (Ren, Ziyan.) | Jia, Ziyue (Jia, Ziyue.) | Wu, Guoding (Wu, Guoding.) | Peng, Yongzhen (Peng, Yongzhen.) (学者:彭永臻)

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EI SCIE

摘要:

Preparing adsorbents with hydrated phosphorophilic metal oxide modified porous materials is a promising method for recovering phosphorus from wastewater. In this study, three kinds of adsorbents were developed by loading iron (), zirconium () and lanthanum () on diatomite under the same preparation conditions (referred to as D-HFO, D-HZO, D-HLO, respectively). The property differences and phosphorus adsorption behavior differences of three adsorbents in actual wastewater were explored. Characterization results indicated that three metals were mainly supported on diatomite in the form of hydrated oxides with nanostructures. In batch experiment, the adsorption capacity of D-HFO, D-HZO was high under acidic conditions, while D-HLO tended to adsorb phosphorus in neutral or slightly alkaline environment. The maximum adsorption capacities of D-HFO, D-HZO, D-HLO to adsorb phosphorus from wastewater were 13.22, 20.25, 148.31 mg/g, respectively. Yet in fixed-bed column experiment, D-HLO particles agglomerated due to its high chemical energy, and the maximum treatment bed-volume (BV) of D-HFO, D-HZO, D-HLO were 120, 315, 210 BV, respectively. Langmuir-Langmuir fitting results showed that the chemical precipitation contribution rate of phosphorus adsorbed on D-HFO, D-HZO, D-HLO was 83.5%, 63.8%, 86.2%, respectively. Ligand exchange and surface complexation were the main recovery mechanisms in phosphorus adsorption process from the actual wastewater by three adsorbents. © 2021 Elsevier B.V.

关键词:

Adsorption Alkalinity Chemicals removal (water treatment) Hydration Metal recovery Metals Phosphorus Porous materials Precipitation (chemical) Secondary recovery

作者机构:

  • [ 1 ] [Li, Shuaishuai]National Engineering Laboratory for Advanced Municipal Wastewater Treatment and Reuse Technology, Beijing University of Technology, Beijing; 100124, China
  • [ 2 ] [Zeng, Wei]National Engineering Laboratory for Advanced Municipal Wastewater Treatment and Reuse Technology, Beijing University of Technology, Beijing; 100124, China
  • [ 3 ] [Ren, Ziyan]National Engineering Laboratory for Advanced Municipal Wastewater Treatment and Reuse Technology, Beijing University of Technology, Beijing; 100124, China
  • [ 4 ] [Jia, Ziyue]National Engineering Laboratory for Advanced Municipal Wastewater Treatment and Reuse Technology, Beijing University of Technology, Beijing; 100124, China
  • [ 5 ] [Wu, Guoding]National Engineering Laboratory for Advanced Municipal Wastewater Treatment and Reuse Technology, Beijing University of Technology, Beijing; 100124, China
  • [ 6 ] [Peng, Yongzhen]National Engineering Laboratory for Advanced Municipal Wastewater Treatment and Reuse Technology, Beijing University of Technology, Beijing; 100124, China

通讯作者信息:

  • 曾薇

    [zeng, wei]national engineering laboratory for advanced municipal wastewater treatment and reuse technology, beijing university of technology, beijing; 100124, china

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来源 :

Colloids and Surfaces A: Physicochemical and Engineering Aspects

ISSN: 0927-7757

年份: 2021

卷: 623

5 . 2 0 0

JCR@2022

ESI学科: CHEMISTRY;

ESI高被引阀值:7

被引次数:

WoS核心集被引频次: 0

SCOPUS被引频次: 9

ESI高被引论文在榜: 0 展开所有

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