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作者:

Hao Zhendong (Hao Zhendong.) | Zhou Ting (Zhou Ting.) | Xiao Tianliang (Xiao Tianliang.) | Gong Hui (Gong Hui.) | Zhang Qianqian (Zhang Qianqian.) | Wang Hao (Wang Hao.) | Zhai Jin (Zhai Jin.)

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摘要:

Nanochannel system provides a promising platform to create nanofluidic components in large-scale integrated circuits for "lab-on-a-chip" applications. However, it is a big challenge to achieve in situ monitoring on microscopic nanofluidic manipulation of single nanofluidic components in the integrated ionic circuit. Herein, we present a simple approach to realize visual nanofluidic manipulation in asymmetric nanochannels by the functionalization of an electrochromic polyaniline coating, which demonstrates redox-tunable surface charge accompanied by a visible color variation. The electrochromic nanochannels present a green color when behaving as ionic diodes, while the color turns to light yellow in a manner of ionic resistor. Moreover, both ionic transport behavior and color transition could respond well with alternating switch between redox states, contributing to a reversible and stable visual nanofluidic manipulation of electrochromic nanochannels. This work will create new avenues on in situ characterizing nanofluidic manipulation of nanofluidic components in integrated ionic circuits for intelligent sensing and detection applications.

关键词:

electrochromism integrated ionic circuits nanochannels

作者机构:

  • [ 1 ] [Hao Zhendong]Key Laboratory for New Functional Materials of Ministry of Education, Faculty of Materials and Manufacturing, Beijing University of Technology, Beijing 100124, P. R. China
  • [ 2 ] [Zhou Ting]Key Laboratory for New Functional Materials of Ministry of Education, Faculty of Materials and Manufacturing, Beijing University of Technology, Beijing 100124, P. R. China
  • [ 3 ] [Xiao Tianliang]Key Laboratory of Bio-Inspired Smart Interfacial Science and Technology of Ministry of Education, School of Chemistry, Beihang University, Beijing 100191, P. R. China
  • [ 4 ] [Gong Hui]Key Laboratory for New Functional Materials of Ministry of Education, Faculty of Materials and Manufacturing, Beijing University of Technology, Beijing 100124, P. R. China
  • [ 5 ] [Zhang Qianqian]Key Laboratory for New Functional Materials of Ministry of Education, Faculty of Materials and Manufacturing, Beijing University of Technology, Beijing 100124, P. R. China
  • [ 6 ] [Wang Hao]Key Laboratory for New Functional Materials of Ministry of Education, Faculty of Materials and Manufacturing, Beijing University of Technology, Beijing 100124, P. R. China
  • [ 7 ] [Zhai Jin]Key Laboratory of Bio-Inspired Smart Interfacial Science and Technology of Ministry of Education, School of Chemistry, Beihang University, Beijing 100191, P. R. China

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来源 :

ACS applied materials & interfaces

ISSN: 1944-8252

年份: 2020

期: 51

卷: 12

页码: 57314-57321

9 . 5 0 0

JCR@2022

ESI学科: MATERIALS SCIENCE;

ESI高被引阀值:169

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WoS核心集被引频次: 0

SCOPUS被引频次: 7

ESI高被引论文在榜: 0 展开所有

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