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作者:

Gaulier, Camille (Gaulier, Camille.) | Zhou, Chunyang (Zhou, Chunyang.) | Gao, Yue (Gao, Yue.) | Guo, Wei (Guo, Wei.) | Reichstadter, Marek (Reichstadter, Marek.) | Ma, Tianhui (Ma, Tianhui.) | Baeyens, Willy (Baeyens, Willy.) | Billon, Gabriel (Billon, Gabriel.)

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摘要:

The biogeochemical behavior of Cd, Co, Cr, Cu, Ni and Pb along the historically polluted Scheldt estuary (Belgium - The Netherlands) was investigated in this study. As never studied before in this area, labile trace metals were measured using the passive sampling technique of Diffusive Gradients in Thin-films (DGT), while total dissolved and particulate trace metal concentrations were assessed using classic active sampling techniques. This dual approach allowed us to highlight the variations of trace metal speciation and distribution in the estuarine surface waters, considering environmental and physicochemical gradients along the transect.The large data set obtained was then compared with literature data of historical measurements along the Scheldt (from 1980 until now), but also from other estuaries. As emphasized by our results, trace metal mobility and partitioning along the Scheldt estuary was mainly driven by biogeochemical reactions which were strongly influenced by gradients of specific estuarine physico-chemical parameters, such as salinity, turbidity, temperature and so on. Hence, all species of trace metals displayed a non-conservative behavior. More precisely, dissolved labile fractions of trace metals showed higher levels in the middle estuary, where many solubilization and remobilization processes occurred due to turbulent mixing mechanisms and an increasing salinity. Our study confirmed the decreasing trend historically observed for particulate metals along the Scheldt, as well as the rising concentrations recorded for dissolved trace metals which might also lead to an increase of their labile fraction measured by the DGT. Finally, these preliminary results suggested that a more regular monitoring of labile metal along the Scheldt estuary is essential to have an in-depth understanding of trace metal speciation and to review bioavailability of trace metals within estuarine ecosystems. (C) 2020 Elsevier B.V. All rights reserved.

关键词:

DGT Non-conservative Trace metal speciation Scheldt estuary Biogeochemical cycle

作者机构:

  • [ 1 ] [Gaulier, Camille]Vrije Univ Brussel, Analyt Environm & Geochem Dept AMGC, Pl Laan 2, B-1050 Brussels, Belgium
  • [ 2 ] [Zhou, Chunyang]Vrije Univ Brussel, Analyt Environm & Geochem Dept AMGC, Pl Laan 2, B-1050 Brussels, Belgium
  • [ 3 ] [Gao, Yue]Vrije Univ Brussel, Analyt Environm & Geochem Dept AMGC, Pl Laan 2, B-1050 Brussels, Belgium
  • [ 4 ] [Guo, Wei]Vrije Univ Brussel, Analyt Environm & Geochem Dept AMGC, Pl Laan 2, B-1050 Brussels, Belgium
  • [ 5 ] [Reichstadter, Marek]Vrije Univ Brussel, Analyt Environm & Geochem Dept AMGC, Pl Laan 2, B-1050 Brussels, Belgium
  • [ 6 ] [Ma, Tianhui]Vrije Univ Brussel, Analyt Environm & Geochem Dept AMGC, Pl Laan 2, B-1050 Brussels, Belgium
  • [ 7 ] [Baeyens, Willy]Vrije Univ Brussel, Analyt Environm & Geochem Dept AMGC, Pl Laan 2, B-1050 Brussels, Belgium
  • [ 8 ] [Gaulier, Camille]Univ Lille, Cite Sci, LASIRE CNRS UMR 8516, F-59655 Villeneuve Dascq, France
  • [ 9 ] [Billon, Gabriel]Univ Lille, Cite Sci, LASIRE CNRS UMR 8516, F-59655 Villeneuve Dascq, France
  • [ 10 ] [Guo, Wei]Beijing Univ Technol, Coll Architecture & Civil Engn, Beijing 100124, Peoples R China
  • [ 11 ] [Reichstadter, Marek]Brno Univ Technol, Fac Chem, Purkynova 118, Brno 62100, Czech Republic

通讯作者信息:

  • [Gao, Yue]Vrije Univ Brussel, Fac Sci, Analyt Environm & Geochem AMGC, Pl Laan 2, B-1050 Brussels, Belgium

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来源 :

SCIENCE OF THE TOTAL ENVIRONMENT

ISSN: 0048-9697

年份: 2021

卷: 757

9 . 8 0 0

JCR@2022

ESI学科: ENVIRONMENT/ECOLOGY;

ESI高被引阀值:94

JCR分区:1

被引次数:

WoS核心集被引频次: 21

SCOPUS被引频次: 26

ESI高被引论文在榜: 0 展开所有

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