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作者:

Zhang, Hanyu (Zhang, Hanyu.) | Xing, Yi (Xing, Yi.) | Cheng, Shuiyuan (Cheng, Shuiyuan.) (学者:程水源) | Wang, Xiaoqi (Wang, Xiaoqi.) | Guan, Panbo (Guan, Panbo.)

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EI Scopus SCIE

摘要:

Characteristics of submicron particulate matter, including its components, during December 5-30, 2016, were comprehensively investigated in Beijing. The surface transport flux was calculated as well as the cross-border transport influence of Beijing and the North China Plain (NCP) on Beijing University of Technology (BJUT) based on the non-refractory submicron particles (NR-PM1) and species, PM2.5, and gaseous pollutant observations, together with wind vectors. The Weather Research & Forecasting (WRF) and Comprehensive Air Quality Model with Extension (CAMx) were applied to demonstrate the vertical PM2.5 flux distribution. These results showed that the monthly average concentration of NR-PM1 was 86.1 +/- 86.5 mu g m(-3), with organics forming the major fraction (49.2 +/- 11.1%), followed by NO3- (19.1 +/- 6.3%), SO42- (15.8 +/- 6.4%), NH4+ (10.8 +/- 2.6%), and Cl (5.1 +/- 2.9%). The accumulation and dissipation of pollutants were related to the wind vector, with higher concentrations in the southern and eastern directions with low wind speed (WS), and lower concentrations in the northwestern direction with high WS. The net flux intensities were stronger from WB to BJUT for particulate matter and species, from EB to BJUT for gaseous pollutants and from NB to BJUT for all pollutants, which might attribute to the mutual influence of the pollutant concentration and wind vector. All the pollutant flux intensities were generally stronger in the heavy pollution episodes (HPEs) and red alert episodes (RAEs) than those in the non-polluted episodes (NPEs). Moreover, the PM2.5 net flux varied with the height; the maximum total net flux occurred at a height of 252 m. The variations in PM2.5 flux at the high-altitude layer were similar to those at the low-altitude layer, in which the former was approximately 1.5-2 times the latter. Furthermore, the external transport could exert important influence before reaching the most severe stage of pollution, while the local emissions had a greater potential to form heavy pollution extremes. Overall, the aforementioned results could provide the scientific support for proposing effective joint control measures and mitigating the adverse effects of heavy pollution in NCP.

关键词:

Heavy pollution Transport flux WRF-CAMx Wind vector impacts NR-PM1

作者机构:

  • [ 1 ] [Zhang, Hanyu]Beijing Univ Technol, Key Lab Beijing Reg Air Pollut Control, Beijing 100124, Peoples R China
  • [ 2 ] [Cheng, Shuiyuan]Beijing Univ Technol, Key Lab Beijing Reg Air Pollut Control, Beijing 100124, Peoples R China
  • [ 3 ] [Wang, Xiaoqi]Beijing Univ Technol, Key Lab Beijing Reg Air Pollut Control, Beijing 100124, Peoples R China
  • [ 4 ] [Guan, Panbo]Beijing Univ Technol, Key Lab Beijing Reg Air Pollut Control, Beijing 100124, Peoples R China
  • [ 5 ] [Zhang, Hanyu]Beijing Technol & Business Univ, Sch Ecol & Environm, Beijing 100048, Peoples R China
  • [ 6 ] [Xing, Yi]Univ Sci & Technol Beijing, Sch Energy & Environm Engn, Beijing 100083, Peoples R China
  • [ 7 ] [Xing, Yi]Univ Sci & Technol Beijing, Beijing Key Lab Resource Oriented Treatment Ind P, Beijing 100083, Peoples R China

通讯作者信息:

  • 程水源

    [Cheng, Shuiyuan]Beijing Univ Technol, Key Lab Beijing Reg Air Pollut Control, Beijing 100124, Peoples R China;;[Xing, Yi]Univ Sci & Technol Beijing, Sch Energy & Environm Engn, Beijing 100083, Peoples R China

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来源 :

ATMOSPHERIC ENVIRONMENT

ISSN: 1352-2310

年份: 2021

卷: 246

5 . 0 0 0

JCR@2022

ESI学科: GEOSCIENCES;

ESI高被引阀值:64

JCR分区:1

被引次数:

WoS核心集被引频次: 8

SCOPUS被引频次: 13

ESI高被引论文在榜: 0 展开所有

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