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作者:

Guo, Wei (Guo, Wei.) | Li, Jun (Li, Jun.) | Liu, Qingwei (Liu, Qingwei.) | Shi, Jianghong (Shi, Jianghong.) | Gao, Yue (Gao, Yue.)

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摘要:

Artificial sweeteners (ASs), as a new emerging pollutant, the fate from wastewater treatment plants (WWTPs) to sea is growing concerned. In this study, the distribution and polluted loading of six typical ASs were analyzed based on the measurement in influent, primary effluent, secondary effluent, tertiary effluent, suspended particulate matter (SPM), and sludge from four WWTPs and receiving waters near the coast of Shenzhen city, China. Elevated levels of ASs were detected in WWTPs located near a highly populated area (about 14,000 people km-2). Sucralose was predominant in all water samples (0.1-22.2 mu g L-1), and had a 1.6-704.0 times higher concentration than the means of other ASs detected. Aspartame were mainly distributed in SPM and sludge, and the fractions in offshore water exceeded 45%. Acesulfame, sucralose, cyclamate and saccharin could be effectively removed by secondary biochemical treatment. The average daily loading (4.2 g d-1 1000people-1) and discharge loading (0.4 g d-1 1000people-1) of sucralose in WWTPs was higher than those of the other ASs. Dissolved organic carbon and UV254 can affect the fate of ASs, and SPM mainly affects the distributions of aspartame and neotame. As a potential sewage indicator, neotame deserves further attention.

关键词:

Artificial sweeteners Mass loading Environmental fate Treatment process Sewage tracers

作者机构:

  • [ 1 ] [Guo, Wei]Beijing Univ Technol, Coll Architecture & Civil Engn, Beijing 100124, Peoples R China
  • [ 2 ] [Li, Jun]Beijing Univ Technol, Coll Architecture & Civil Engn, Beijing 100124, Peoples R China
  • [ 3 ] [Liu, Qingwei]Southern Univ Sci & Technol, Sch Environm Sci & Engn, State Environm Protect Key Lab Integrated Surface, Shenzhen 518055, Peoples R China
  • [ 4 ] [Shi, Jianghong]Southern Univ Sci & Technol, Sch Environm Sci & Engn, State Environm Protect Key Lab Integrated Surface, Shenzhen 518055, Peoples R China
  • [ 5 ] [Gao, Yue]Vrije Univ Brussel VUB, Analyt Environm & Geochem AMGC, B-1050 Brussels, Belgium

通讯作者信息:

  • [Guo, Wei]Beijing Univ Technol, Coll Architecture & Civil Engn, Beijing 100124, Peoples R China

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来源 :

JOURNAL OF HAZARDOUS MATERIALS

ISSN: 0304-3894

年份: 2021

卷: 414

1 3 . 6 0 0

JCR@2022

ESI学科: ENGINEERING;

ESI高被引阀值:87

JCR分区:1

被引次数:

WoS核心集被引频次: 23

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ESI高被引论文在榜: 0 展开所有

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