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We have prepared GexSe10Te90-x glasses with a composition of x from 17.5 to 26.25 and measured their properties using various diagnosis tools. It was found that, all the glasses have a transmittance more than 40% at a wavelength range from 2 to 15 mu m, and linear refractive index n0 decreases but optical bandgap energy Eg increases with decreasing Te contents in the glasses. We also analysed the evolution of n2 and beta as a function of Ge content, both the evolution of n2 and beta are close to the prediction by Sheik-Bahae et al. for optical nonlinearity of semiconductors. In all cases, the nonlinear optical refractive index n2 measured at 3.0 mu m is larger than that at 2.5 mu m due to the two-photon resonance effect, and a maximum nonlinear index is 2.46 x 10-13 cm2/W at composition of Ge17.5Se10Te72.5. Such larger nonlinearity around 10-13 cm2/W observed in the present paper is one order of the magnitude larger than that in S- and Se-based chalcogenide glasses, demonstrating potentials of Te-based glasses for the applications as mid- and far-infrared nonlinear optical devices.
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