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作者:

Yao, Sen (Yao, Sen.) | Wang, Qianheng (Wang, Qianheng.) | Zhang, Junmei (Zhang, Junmei.) | Zhang, Ruinan (Zhang, Ruinan.)

收录:

SCIE

摘要:

In order to investigate the chemical characteristics of aerosol pollution including PM1 and PM2.5 in Handan, the offline sampling campaign was conducted and the concentrations of total water-soluble inorganic ions (TWSI), carbonaceous components (OC and EC) were analyzed. The average concentrations were 88.5 mu g/m(3) for PM1 and 122 mu g/m(3) for PM2.5, and the corresponding ratios of PM1 versus PM2.5 on non-pollution, mild-moderate pollution and heavy pollution were 0.67, 0.70 and 0.77, respectively. TWSI and OC accounted for 43.2% and 15.4% in PM1, 41.8% and 16.0% in PM2.5. Secondary components in PM2.5 and PM1 increased with heavy pollution, SNA (SO42-, NO3- and NH4+) was enriched in PM1 but SOC (Secondary Organic Carbon) was more enriched in PM1-2.5. Furthermore, for evaluating the effect of aerosol feedback the WRF-Chem model was applied to identify the aerosol-radiation interaction of aerosol feedback influence on the PM2.5 concentration and various meteorological factors in Handan. The results indicated that the aerosol radiative effects will result in an average 32.62%(36.18 W/m(2)) decrease in downward short wave flux at ground surface (SWDOWN), an average 17.52% (39.15 m) and 0.16% (0.44 K) decrease in planetary boundary layer height(PBLH) and surface temperature (T2). The wind speed at 10 m (WS) and relative humidity (RH) will be increased by about 4.16%(0.11 m/s) and 1.89% (0.78%), respectively.

关键词:

5 aerosol feedback carbonaceous components PM1 PM2 water soluble inorganic ions

作者机构:

  • [ 1 ] [Yao, Sen]Zhongyuan Univ Technol, Sch Energy & Environm, Zhengzhou 450007, Peoples R China
  • [ 2 ] [Wang, Qianheng]Zhongyuan Univ Technol, Sch Energy & Environm, Zhengzhou 450007, Peoples R China
  • [ 3 ] [Zhang, Junmei]Zhongyuan Univ Technol, Sch Energy & Environm, Zhengzhou 450007, Peoples R China
  • [ 4 ] [Zhang, Ruinan]Zhongyuan Univ Technol, Sch Energy & Environm, Zhengzhou 450007, Peoples R China
  • [ 5 ] [Yao, Sen]Beijing Univ Technol, Key Lab Beijing Reg Air Pollut Control, Beijing 100124, Peoples R China

通讯作者信息:

  • [Yao, Sen]Zhongyuan Univ Technol, Sch Energy & Environm, Zhengzhou 450007, Peoples R China;;[Yao, Sen]Beijing Univ Technol, Key Lab Beijing Reg Air Pollut Control, Beijing 100124, Peoples R China

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来源 :

ATMOSPHERE

年份: 2021

期: 6

卷: 12

2 . 9 0 0

JCR@2022

ESI学科: GEOSCIENCES;

ESI高被引阀值:6

被引次数:

WoS核心集被引频次: 1

SCOPUS被引频次: 3

ESI高被引论文在榜: 0 展开所有

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