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作者:

Zhao, Na (Zhao, Na.) | Wang, Gang (Wang, Gang.) | Li, Guohao (Li, Guohao.) | Lang, Jianlei (Lang, Jianlei.) (学者:郎建垒)

收录:

SCIE

摘要:

Although weather conditions significantly affect air pollutant concentrations, few quantitative studies have been conducted on the effects of long-term and seasonal changes in meteorology on air quality. Hence, in this study, the trends in Shandong Province, China, for six criteria pollutants (viz., sulfur dioxide [SO2], carbon monoxide [CO], particulate matter [PM] with an aerodynamic diameter of < 10 mu m [PM10], PM with an aerodynamic diameter of < 2.5 mu m [PM2.5], nitrogen dioxide [NO2], and ozone [O-3]) were analyzed for the period of 2013-2019, when overall emissions of air pollutants decreased, and the Weather Research and Forecasting model coupled with Chemistry (WRF/Chem) was applied to evaluate the role of inter-annual and seasonal meteorological changes. Five of the six criteria pollutants exhibited a sharp drop in concentration until 2017 and a gradual decline afterward, with the maximum and minimum annual values occurring during winter and summer, respectively. In contrast, the level of O-3 rose between 2013 and 2019 and displayed the opposite seasonal trend. Also, the diurnal concentrations of the first five criteria pollutants showed a typical bimodal distribution, whereas those of the O-3 showed a typical unimodal distribution. Furthermore, a trimodal distribution was observed for the ratios between the diurnal PM2.5 and PM10 concentrations. Using 2013 as the baseline, the inter-annual meteorological changes accounted for only 3.4-18.6% of the decrease in the five criteria pollutants-with little effect on the O-3-between 2015 and 2019, indicating that emission control measures drove the long-term improvement in air quality during these years. However, seasonal meteorological factors, which favored diffusion during summer and winter but accumulation during spring and autumn, played a larger role in the short term for all six species, especially during winter, when they reduced concentrations (excluding those of SO2 in 2019 and O-3 altogether) by 6.5-31.0%.

关键词:

Air pollution Diurnal variation Meteorological condition Seasonal variation WRF/Chem

作者机构:

  • [ 1 ] [Zhao, Na]Fudan Univ, Inst Atmospher Sci, Dept Environm Sci & Engn, Shanghai Key Lab Atmospher Particle Pollut & Prev, Shanghai 200433, Peoples R China
  • [ 2 ] [Wang, Gang]East China Normal Univ, Shanghai Key Lab Urban Ecol Proc & Ecorestorat, Shanghai 200241, Peoples R China
  • [ 3 ] [Wang, Gang]China Univ Petr East China, Coll Chem Engn, Dept Environm & Safety Engn, Qingdao 266580, Peoples R China
  • [ 4 ] [Li, Guohao]Municipal Res Inst Environm Protect, Beijing 100037, Peoples R China
  • [ 5 ] [Li, Guohao]Key Lab Beijing VOC Pollut Control Technol & Appl, Beijing 100037, Peoples R China
  • [ 6 ] [Lang, Jianlei]Beijing Univ Technol, Key Lab Beijing Reg Air Pollut Control, Beijing 100124, Peoples R China

通讯作者信息:

  • 郎建垒

    [Wang, Gang]East China Normal Univ, Shanghai Key Lab Urban Ecol Proc & Ecorestorat, Shanghai 200241, Peoples R China;;[Wang, Gang]China Univ Petr East China, Coll Chem Engn, Dept Environm & Safety Engn, Qingdao 266580, Peoples R China;;[Lang, Jianlei]Beijing Univ Technol, Key Lab Beijing Reg Air Pollut Control, Beijing 100124, Peoples R China

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来源 :

AEROSOL AND AIR QUALITY RESEARCH

ISSN: 1680-8584

年份: 2021

期: 6

卷: 21

4 . 0 0 0

JCR@2022

ESI学科: ENVIRONMENT/ECOLOGY;

ESI高被引阀值:7

被引次数:

WoS核心集被引频次: 14

SCOPUS被引频次: 14

ESI高被引论文在榜: 0 展开所有

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