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作者:

Wang, Xiaoqi (Wang, Xiaoqi.) | Wei, Wei (Wei, Wei.) | Cheng, Shuiyuan (Cheng, Shuiyuan.) (学者:程水源) | Wang, Ruipeng (Wang, Ruipeng.) | Zhu, Jiaxian (Zhu, Jiaxian.)

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Scopus SCIE

摘要:

Beijing has achieved significant air quality improvement over the past decade. In this study, we applied a simulation technique on pollutant monitoring data to investigate the contribution of emission reduction (ERE) and meteorological effects (ME) to the improvement of air quality. We measured the daily PM2.5 concentrations during four months (representing the four seasons) in 2013 and 2018. We found that the concentrations of NH4+, NO3, and SO42- decreased from 2013 to 2018, but the proportion of NO3 in PM2.5 showed an apparent increase. Multiple scenarios were simulated using the WRF-CAMx model to determine the impact of ERE and ME on air pollution. The results showed that both variables positively contributed to the annual air quality improvement, with ERE contributing more than 70% to the total PM2.5 reduction. However, their seasonal contributions showed notable differences. In winter, ME contributed more than 40 mu g/m(3) to the PM2.5 decrease, which was much higher than that in other seasons. This suggests that the positive effect of pollutant emission reduction on air quality may have been weakened under extremely adverse meteorological conditions. Hence, the monitoring and modeling results were coupled to evaluate the secondary conversion degree. We found that the emissions of precursors, including SO2 and NOx, notably decreased, but both the local and regional conversion degrees increased from 2013 to 2018. Therefore, for effective air pollution reduction, we suggest that future air pollution mitigation measures should focus on reducing secondary pollution in Beijing.

关键词:

Secondary conversion degree Emission reduction effect Meteorological effect Air quality improvement

作者机构:

  • [ 1 ] [Wang, Xiaoqi]Beijing Univ Technol, Key Lab Beijing Reg Air Pollut Control, Beijing 100124, Peoples R China
  • [ 2 ] [Wei, Wei]Beijing Univ Technol, Key Lab Beijing Reg Air Pollut Control, Beijing 100124, Peoples R China
  • [ 3 ] [Cheng, Shuiyuan]Beijing Univ Technol, Key Lab Beijing Reg Air Pollut Control, Beijing 100124, Peoples R China
  • [ 4 ] [Wang, Ruipeng]Beijing Univ Technol, Key Lab Beijing Reg Air Pollut Control, Beijing 100124, Peoples R China
  • [ 5 ] [Zhu, Jiaxian]Beijing Univ Technol, Key Lab Beijing Reg Air Pollut Control, Beijing 100124, Peoples R China

通讯作者信息:

  • [Wei, Wei]Beijing Univ Technol, Key Lab Beijing Reg Air Pollut Control, Beijing 100124, Peoples R China

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来源 :

ATMOSPHERIC POLLUTION RESEARCH

ISSN: 1309-1042

年份: 2021

期: 5

卷: 12

4 . 5 0 0

JCR@2022

ESI学科: ENVIRONMENT/ECOLOGY;

ESI高被引阀值:94

JCR分区:2

被引次数:

WoS核心集被引频次: 7

SCOPUS被引频次: 11

ESI高被引论文在榜: 0 展开所有

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