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作者:

Li, Sumei (Li, Sumei.) | Feng, Fan (Feng, Fan.) | Chen, Sha (Chen, Sha.) (学者:陈莎) | Zhang, Xiaolei (Zhang, Xiaolei.) | Liang, Yixuan (Liang, Yixuan.) | Shan, Saisai (Shan, Saisai.)

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摘要:

MOFs are usually used as efficient adsorbents to remove specific pollutants in water. However, because of their poor water stability relatively small particle size, their application in adsorbing and removing pollutants from water is limited. In this paper, with nitrile rubber sponge as the substrate, UiO-66-NH2/sponge composites were firstly in -situ synthesized and systematically evaluated UiO-66-NH2 as an adsorbent to remove 2,4-dichlorophenoxyacetic acid from water. This composite could not only remain the adsorption capacity for 2,4-dichlorophenoxyacetic acid of UiO-66-NH2, but also was much more convenient for separation after the adsorption compared to UIO-66-NH2. In addition, the mechanism of the adsorption of UiO-66-NH2 for 2,4-dichlorophenoxyacetic acid were discussed in detail. Electrostatic interaction between UIO-66-NH2 and 2,4-dichlorophenoxyacetic acid was the main adsorption mechanism. The adsorption was mainly suitable for Langmuir isotherm models, and its maximum adsorption capacity of 2,4-dichlorophenoxyacetic acid was 72.99 mg g(-1).

关键词:

2,4-Dichlorophenoxyacetic acid Metal organic frameworks MOF composites Adsorption

作者机构:

  • [ 1 ] [Li, Sumei]Beijing Univ Technol, Key Lab Beijing Reg Air Pollut Control, Coll Environm & Energy Engn, Beijing 100124, Peoples R China
  • [ 2 ] [Feng, Fan]Beijing Univ Technol, Key Lab Beijing Reg Air Pollut Control, Coll Environm & Energy Engn, Beijing 100124, Peoples R China
  • [ 3 ] [Chen, Sha]Beijing Univ Technol, Key Lab Beijing Reg Air Pollut Control, Coll Environm & Energy Engn, Beijing 100124, Peoples R China
  • [ 4 ] [Liang, Yixuan]Beijing Univ Technol, Key Lab Beijing Reg Air Pollut Control, Coll Environm & Energy Engn, Beijing 100124, Peoples R China
  • [ 5 ] [Shan, Saisai]Beijing Univ Technol, Key Lab Beijing Reg Air Pollut Control, Coll Environm & Energy Engn, Beijing 100124, Peoples R China
  • [ 6 ] [Zhang, Xiaolei]Beijing Univ Technol, Coll Environm & Energy Engn, Beijing Key Lab Green Catalysis & Separat, Beijing 100124, Peoples R China
  • [ 7 ] [Zhang, Xiaolei]Beijing Univ Technol, Coll Environm & Energy Engn, Dept Chem & Chem Engn, Beijing 100124, Peoples R China

通讯作者信息:

  • 陈莎

    [Chen, Sha]Beijing Univ Technol, Key Lab Beijing Reg Air Pollut Control, Coll Environm & Energy Engn, Beijing 100124, Peoples R China

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来源 :

ECOTOXICOLOGY AND ENVIRONMENTAL SAFETY

ISSN: 0147-6513

年份: 2020

卷: 194

6 . 8 0 0

JCR@2022

ESI学科: ENVIRONMENT/ECOLOGY;

ESI高被引阀值:138

被引次数:

WoS核心集被引频次: 51

SCOPUS被引频次: 52

ESI高被引论文在榜: 0 展开所有

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