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作者:

Zhong, Yisheng (Zhong, Yisheng.) | Wang, Xiaoqi (Wang, Xiaoqi.) | Cheng, Shuiyuan (Cheng, Shuiyuan.) (学者:程水源)

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EI Scopus SCIE

摘要:

Beijing, the capital city of China, has achieved remarkable progress in terms of an improvement in air quality under strict control policies in the past 10 years from various sources. In this paper, the characteristics of fine particulate matter (PM2.5) and O-3 in January 2013 and 2018 in Beijing are discussed on the basis of daily sample analysis and hourly monitoring data. It was found that the PM2.5 pollution for the month of January in Beijing has been greatly curbed. The SO42- concentration and proportion of PM2.5 decreased, while the proportions of NO3- and NH4+ increased. Organic matter represented the major component during the two periods with the proportions of 31.7% +/- 8.2% and 31.4% +/- 9.8%. The results of the Hybrid Single Particle Lagrangian Integrated Trajectory (Hysplit) model and Potential Source Contribution Function (PSCF) method showed that air mass from southern nearby regions accounted for 34% and 10% in 2013 and 2018, respectively, which was closely related to the pollution period. Thus, the input direction of air mass in January 2018 was more conducive to the diffusion of pollutants. Modeling results of the Weather Research and Forecasting model (WRF) coupled with Comprehensive Air Quality Model Extensions (CAMx) indicated that the contribution of industry sources to PM2.5 and O-3 decreased from 2013 to 2018, while mobile sources increased. This was mainly due to the different control policies on various emission sources. In terms of O-3 sources, more control measurements should be taken on volatile organic compounds (VOCs) due to its prominent effect on O-3 concentration in both periods. The reduction in emissions and the meteorological conditions both contributed effectively to the sharp decrease in PM2.5 concentration. However, the change in weather conditions had the greater impact on the decrease in PM2.5 concentration, while the reduction in emissions was weakened as a function of this change.

关键词:

PM2.5 chemical components source apportionment O-3 potential source

作者机构:

  • [ 1 ] [Zhong, Yisheng]Beijing Univ Technol, Key Lab Beijing Reg Air Pollut Control, Beijing 100124, Peoples R China
  • [ 2 ] [Wang, Xiaoqi]Beijing Univ Technol, Key Lab Beijing Reg Air Pollut Control, Beijing 100124, Peoples R China
  • [ 3 ] [Cheng, Shuiyuan]Beijing Univ Technol, Key Lab Beijing Reg Air Pollut Control, Beijing 100124, Peoples R China

通讯作者信息:

  • [Wang, Xiaoqi]Beijing Univ Technol, Key Lab Beijing Reg Air Pollut Control, Beijing 100124, Peoples R China

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来源 :

ATMOSPHERE

年份: 2020

期: 12

卷: 11

2 . 9 0 0

JCR@2022

ESI学科: GEOSCIENCES;

ESI高被引阀值:99

被引次数:

WoS核心集被引频次: 8

SCOPUS被引频次: 8

ESI高被引论文在榜: 0 展开所有

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