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作者:

Zeng, Huiping (Zeng, Huiping.) | Wang, Fanshuo (Wang, Fanshuo.) | Xu, Ke (Xu, Ke.) | Zhang, Jie (Zhang, Jie.) | Li, Dong (Li, Dong.) (学者:李冬)

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EI SCIE

摘要:

The porosity of Chitosan Alginate Fe-sludge Beads strengthened with manganese sludge (CAFBs) was optimized by adding CaCO3 or NaHCO3 powder to generate CO2 gas during the preparation process. Two types of adsorbent Dropped-CAFBs (D-CAFBs) and Heated-CAFBs (H-CAFBs) were made. SEM-EDS, BET, XRD as well as adsorption kinetics and isothermal adsorption experiments were used to evaluate the effects of the two pore-forming methods. The SEM-EDS, BET results confirmed that the prepared adsorbent has good porosity and specific surface area was 128.16m2/g. XRD results showed that the structure is amorphous iron manganese oxide. The pseudo-second, intra-particle and Freundlich model were suitable to describe the adsorption process(R2>0.9), the maximum adsorption capacity of As(III) at 298K is 24.06mg/g. The experiments indicate the pH ranging from 9 to 10 and the air aeration intensity adjusted to 1L/min is favorable for regeneration, the percent of As(III) removal is as high as about 80% after 4 adsorption-desorption cycles. © 2020 Elsevier B.V.

关键词:

Adsorption Calcite Calcium carbonate Chitosan Iron metallography Iron oxides Manganese metallography Manganese oxide Pollution control Porosity Sodium bicarbonate X ray diffraction

作者机构:

  • [ 1 ] [Zeng, Huiping]Key Laboratory of Water Quality Science and Water Environment Recovery Engineering, Beijing University of Technology, Beijing; 100124, China
  • [ 2 ] [Wang, Fanshuo]Key Laboratory of Water Quality Science and Water Environment Recovery Engineering, Beijing University of Technology, Beijing; 100124, China
  • [ 3 ] [Xu, Ke]Key Laboratory of Water Quality Science and Water Environment Recovery Engineering, Beijing University of Technology, Beijing; 100124, China
  • [ 4 ] [Zhang, Jie]Key Laboratory of Water Quality Science and Water Environment Recovery Engineering, Beijing University of Technology, Beijing; 100124, China
  • [ 5 ] [Zhang, Jie]State Key Laboratory of Urban Water Resource and Environment, Harbin Institute of Technology, Harbin; 150090, China
  • [ 6 ] [Li, Dong]Key Laboratory of Water Quality Science and Water Environment Recovery Engineering, Beijing University of Technology, Beijing; 100124, China

通讯作者信息:

  • 李冬

    [li, dong]key laboratory of water quality science and water environment recovery engineering, beijing university of technology, beijing; 100124, china

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来源 :

Colloids and Surfaces A: Physicochemical and Engineering Aspects

ISSN: 0927-7757

年份: 2020

卷: 607

5 . 2 0 0

JCR@2022

ESI学科: CHEMISTRY;

ESI高被引阀值:33

JCR分区:2

被引次数:

WoS核心集被引频次: 0

SCOPUS被引频次: 28

ESI高被引论文在榜: 0 展开所有

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