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[期刊论文]

Large electrocaloric strength in Bi(Mg0.5Ti0.5)O-3-modified tetragonal- structured Bi0.5Na0.5TiO3-12.5BaTiO(3) ceramics

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作者:

Zhu, Mankang (Zhu, Mankang.) | Yan, Xiaofen (Yan, Xiaofen.) | Wei, Qiumei (Wei, Qiumei.) | 展开

收录:

EI Scopus SCIE

摘要:

Taking the advantage of the low transition barrier between P4bm and P4mm distortions, tetragonal structured 0.875Bi(0.5)Na(0.5)TiO(3)-0.125BaTiO(3) was designed to construct an electrocaloric ceramics with large electrocaloric strength by adding the third compound Bi(Mg0.5Ti0.5)O-3 (BMT). The experiments show that, through adding 2.5 mol.% BMT, a large Delta T of 0.80 K was directly observed under 4 kV/mm; especially, a high Delta T/Delta E of 0.020-0.023 K cm/kV was achieved, approximate to BaTiO3-based and some lead-based relaxors. The high electrocaloric effect is attributed to that the 2.5 mol.% BMT added sample bridges the nonergodic ferroelectric and ergodic relaxor states, and exhibits a microstructure coexisting P4bm and P4mm symmetries. Our design provides a new route in probing lead-free BNT-based electrocaloric materials apart from the MPB. (C) 2021 Elsevier B.V. All rights reserved.

关键词:

Bismuth sodium titanate Tetragonal distortion Ferroelectric-to-relaxor transition Electrocaloric effect Dynamics of polar nanoregions

作者机构:

  • [ 1 ] [Zhu, Mankang]Beijing Univ Technol, Fac Mat & Mfg, Minist Educ, Key Lab Adv Funct Mat, Beijing 100124, Peoples R China
  • [ 2 ] [Yan, Xiaofen]Beijing Univ Technol, Fac Mat & Mfg, Minist Educ, Key Lab Adv Funct Mat, Beijing 100124, Peoples R China
  • [ 3 ] [Wei, Qiumei]Beijing Univ Technol, Fac Mat & Mfg, Minist Educ, Key Lab Adv Funct Mat, Beijing 100124, Peoples R China
  • [ 4 ] [Zheng, Mupeng]Beijing Univ Technol, Fac Mat & Mfg, Minist Educ, Key Lab Adv Funct Mat, Beijing 100124, Peoples R China
  • [ 5 ] [Hou, Yudong]Beijing Univ Technol, Fac Mat & Mfg, Minist Educ, Key Lab Adv Funct Mat, Beijing 100124, Peoples R China
  • [ 6 ] [Ke, Xiaoxing]Beijing Univ Technol, Inst Microstruct & Properties Adv Mat, Beijing 100124, Peoples R China
  • [ 7 ] [Bai, Yang]Univ Sci & Technol Beijing, Inst Adv Mat & Technol, Beijing Adv Innovat Ctr Mat Genome Engn, Beijing 100083, Peoples R China

通讯作者信息:

  • [Zhu, Mankang]Beijing Univ Technol, Fac Mat & Mfg, Minist Educ, Key Lab Adv Funct Mat, Beijing 100124, Peoples R China;;[Ke, Xiaoxing]Beijing Univ Technol, Inst Microstruct & Properties Adv Mat, Beijing 100124, Peoples R China

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来源 :

JOURNAL OF ALLOYS AND COMPOUNDS

ISSN: 0925-8388

年份: 2021

卷: 889

6 . 2 0 0

JCR@2022

ESI学科: MATERIALS SCIENCE;

ESI高被引阀值:116

JCR分区:1

被引次数:

WoS核心集被引频次: 6

SCOPUS被引频次: 5

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