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作者:

Li, Shuaishuai (Li, Shuaishuai.) | Zeng, Wei (Zeng, Wei.) (学者:曾薇) | Ren, Ziyan (Ren, Ziyan.) | Jia, Ziyue (Jia, Ziyue.) | Peng, Xiaojing (Peng, Xiaojing.) | Peng, Yongzhen (Peng, Yongzhen.) (学者:彭永臻)

收录:

SCIE

摘要:

As a promising phosphorus source, phosphorus recovery from sewage sludge ash is necessary to ensure sustainable phosphorus cycle and management. To achieve these targets, a novel strategy including phosphorus capture by acid-resistant adsorbent from acid-extract of sewage sludge ash and repeated enrichment in eluent was first proposed in this study. Over 93% of phosphorus was extracted by H2SO4 acidification at pH of 2.0, and a tailored acid-resistant adsorbent recovered almost all the extracted phosphorus in acid-extract of sewage sludge ash. The fitting results of multiple models showed that the rate-limiting step for phosphorus recovery was chemical reaction, and the maximum recovery capacity of acid-resistant adsorbent was 41.7-44.0 mg/g. Characterization results of X-ray photoelectron spectroscopy, Fourier transform infrared spectroscopy and Zeta potential suggested that the recovery mechanism of acid-resistant adsorbent for phosphorus included ligand exchange, inner-sphere complexation and electrostatic attraction. After 8 cycles of recovery-repeated enrichment, the phosphorus in eluent was enriched about 6.7 times. Over 99% of phosphorus in eluent was recovered as struvite by adding external magnesium and ammonium at pH of 8.5. The content of heavy metals in recovered struvite were far below the utilization standard of plant fertilizer, indicating that the phosphorus in sewage sludge ash could be recovered in the form of high-quality phosphorus fertilizer.

关键词:

Acid-resistant adsorbent Phosphorus recovery Repeated enrichment Sewage sludge ash Struvite

作者机构:

  • [ 1 ] [Li, Shuaishuai]Beijing Univ Technol, Natl Engn Lab Adv Municipal Wastewater Treatment, Beijing 100124, Peoples R China
  • [ 2 ] [Zeng, Wei]Beijing Univ Technol, Natl Engn Lab Adv Municipal Wastewater Treatment, Beijing 100124, Peoples R China
  • [ 3 ] [Ren, Ziyan]Beijing Univ Technol, Natl Engn Lab Adv Municipal Wastewater Treatment, Beijing 100124, Peoples R China
  • [ 4 ] [Jia, Ziyue]Beijing Univ Technol, Natl Engn Lab Adv Municipal Wastewater Treatment, Beijing 100124, Peoples R China
  • [ 5 ] [Peng, Xiaojing]Beijing Univ Technol, Natl Engn Lab Adv Municipal Wastewater Treatment, Beijing 100124, Peoples R China
  • [ 6 ] [Peng, Yongzhen]Beijing Univ Technol, Natl Engn Lab Adv Municipal Wastewater Treatment, Beijing 100124, Peoples R China

通讯作者信息:

  • 曾薇

    [Zeng, Wei]Beijing Univ Technol, Dept Environm Engn, Pingleyuan 100, Beijing 100124, Peoples R China

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来源 :

JOURNAL OF CLEANER PRODUCTION

ISSN: 0959-6526

年份: 2021

卷: 322

1 1 . 1 0 0

JCR@2022

ESI学科: ENGINEERING;

ESI高被引阀值:9

被引次数:

WoS核心集被引频次: 11

SCOPUS被引频次: 12

ESI高被引论文在榜: 0 展开所有

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中文被引频次:

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