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作者:

Wu, Jin (Wu, Jin.) | Li, Jiao (Li, Jiao.) | Teng, Yanguo (Teng, Yanguo.) | Chen, Haiyang (Chen, Haiyang.) | Wang, Yeyao (Wang, Yeyao.)

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摘要:

Apportion soil heavy metal sources across large-scale regions is a challenging task. The present study developed a modified receptor model to estimate the contributions of various sources to soil heavy metals and the associated health risks at a large scale. A positive matrix factorization model based on a partition computing approach was employed; the entire study area was divided into several zones for the source apportionment and then calculated together, termed partition computing-PMF (PC-PMF). The agricultural soil in Tianjin, China, was chosen for the case study. The PC-PMF results showed that irrigation, atmospheric deposition and sludge application were the main anthropogenic sources, with contributions of 26.60 %, 19.56 % and 2.86 %, respectively. We subsequently combined PC-PMF with a human health risk assessment model (HHRA) to obtain the human health risk of every source category. The natural background was regarded as a major factor influencing human health in the study area, with contributions of 38.03 % for the noncarcinogenic risk and 28.68 % for the carcinogenic risk. The results indicated that PC-PMF performed better at the source apportionment of soil heavy metals than PMF. This study provides a good example of how the spatial variability can be utilized to reduce the uncertainty in source apportionment.

关键词:

Agricultural soil heavy metals Human health risk Positive matrix factorization Source apportionment Spatial distribution

作者机构:

  • [ 1 ] [Wu, Jin]Beijing Univ Technol, Coll Architecture & Civil Engn, Beijing 100124, Peoples R China
  • [ 2 ] [Li, Jiao]Chinese Res Inst Environm Sci, Beijing 100012, Peoples R China
  • [ 3 ] [Li, Jiao]Minist Ecol & Environm, Tech Ctr Soil Agr & Rural Ecol & Environm, Beijing 100012, Peoples R China
  • [ 4 ] [Teng, Yanguo]Beijing Normal Univ, Coll Water Sci, Beijing 100875, Peoples R China
  • [ 5 ] [Chen, Haiyang]Beijing Normal Univ, Coll Water Sci, Beijing 100875, Peoples R China
  • [ 6 ] [Wang, Yeyao]China Natl Environm Monitoring Ctr, Beijing 100012, Peoples R China

通讯作者信息:

  • [Li, Jiao]Minist Ecol & Environm, Tech Ctr Soil Agr & Rural Ecol & Environm, Beijing 100012, Peoples R China;;[Teng, Yanguo]Beijing Normal Univ, Coll Water Sci, Beijing 100875, Peoples R China

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来源 :

JOURNAL OF HAZARDOUS MATERIALS

ISSN: 0304-3894

年份: 2020

卷: 388

1 3 . 6 0 0

JCR@2022

ESI学科: ENGINEERING;

ESI高被引阀值:28

JCR分区:1

被引次数:

WoS核心集被引频次: 156

SCOPUS被引频次: 121

ESI高被引论文在榜: 0 展开所有

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