A　facile　and　effective　method　to　fabricate　highly　pseudocapacitive　electrodes　of　Fe-Ti-O@C　has　been　proposed　here.　In　this　strategy,　FeOOH　crystals　were　firstly　grown　uniformly　on　the　surface　of　Ti-based　MOF　(MIL-125)　tablet　substrates　through　a　solution　immersion　method,　and　then　converted　to　uniform　carbon　supported　Fe-Ti-O　composites　by　calcination　under　argon.　The　obtained　Fe-Ti-O@C　composites　were　first　utilized　as　an　efficient　anode　for　lithium　ion　batteries　with　a　high　reversible　capacity　of　988　mA　h　g(-1)　after　160　cycles　at　200　mA　g(-1).　Such　a　superior　lithium　storage　performance　may　be　due　to　the　synergistic　effect　of　the　Fe3O4　nanoparticles　with　a　high　capacity,　FeTiO3　nanocomposites　with　a　nearly　stable　structure　during　the　Li+　insertion/removal　process,　and　the　conductive　carbon　skeleton　with　a　large　surface　area　and　porous　structure.　This　work　represents　an　important　step　forward　in　the　fabrication　of　MOF-derived　hybrids　and　enables　transition　metal　oxides　(TMOs)　to　have　potential　applications　in　energy　storage　systems.