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作者:

Ou, Shengju (Ou, Shengju.) | Wei, Wei (Wei, Wei.) | Cheng, Shuiyuan (Cheng, Shuiyuan.) | Cai, Bin (Cai, Bin.)

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EI Scopus SCIE

摘要:

Continuous aggravated surface O-3 over North China Plain (NCP) has attracted widely public concern. Herein, we evaluated the effects of changes in aerosols, precursor emissions, and meteorology on O-3 in summer (June) of 2015-2019 over NCP via 8 scenarios with WRF-Chem model. The simulated mean MDA8 O-3 in urban areas of 13 major cities in NCP increased by 17.1%similar to 34.8%, which matched well with the observations (10.8%similar to 33.1%). Meanwhile, the model could faithfully reproduce the changes in aerosol loads, precursors, and meteorological conditions. A relatively-even O-3 increase (+1.2%similar to+3.9% for 24-h O-3 and +1.0%similar to+3.8% for MDA8 O-3) was induced by PM2.5 dropping, which was consistent with the geographic distribution of regional PM2.5 reduction. Meanwhile, the NO2 reduction coupled with a near-constant VOCs led to the elevated VOCs/NOx ratios, and then caused O-3 rising in the areas under VOCs-limited regimes. Therein, the pronounced increases occurred in Handan, Xingtai, Shijiazhuang, Tangshan, and Langfang (+10.7%similar to+13.6% for 24-h O-3 and +10.2%similar to+12.2% for MDA8 O-3); while the increases in other cities were 5.7%similar to 10.5% for 24-h O-3 and 4.9%similar to 9.2% for MDA8 O-3. Besides, the meteorological fluctuations brought about the more noticeable O-3 increases in northern parts (+12.5%similar to+13.5% for 24-h O-3 and +11.2%similar to+12.4% for MDA8 O-3) than those in southern and central parts (+3.2%similar to+9.3% for 24-h O-3 and +3.7%similar to+8.8% for MDA8 O-3). The sum of the impacts of the three drivers reached 16.7%similar to 21.9%, which were comparable to the changes of the observed O-3. Therefore, exploring reasonable emissions-reduction strategies is essential for the ozone pollution mitigation over this region. (C) 2022 The Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences. Published by Elsevier B.V.

关键词:

Precursors Meteorology WRF-Chem model Aerosols Surface ozone Driving force

作者机构:

  • [ 1 ] [Ou, Shengju]Beijing Univ Technol, Fac Environm & Life, Key Lab Beijing Reg Air Pollut Control, Beijing 100124, Peoples R China
  • [ 2 ] [Wei, Wei]Beijing Univ Technol, Fac Environm & Life, Key Lab Beijing Reg Air Pollut Control, Beijing 100124, Peoples R China
  • [ 3 ] [Cheng, Shuiyuan]Beijing Univ Technol, Fac Environm & Life, Key Lab Beijing Reg Air Pollut Control, Beijing 100124, Peoples R China
  • [ 4 ] [Cai, Bin]Beijing Univ Technol, Fac Environm & Life, Key Lab Beijing Reg Air Pollut Control, Beijing 100124, Peoples R China

通讯作者信息:

  • [Wei, Wei]Beijing Univ Technol, Fac Environm & Life, Key Lab Beijing Reg Air Pollut Control, Beijing 100124, Peoples R China;;[Cheng, Shuiyuan]Beijing Univ Technol, Fac Environm & Life, Key Lab Beijing Reg Air Pollut Control, Beijing 100124, Peoples R China;;

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来源 :

JOURNAL OF ENVIRONMENTAL SCIENCES

ISSN: 1001-0742

年份: 2023

卷: 127

页码: 453-464

6 . 9 0 0

JCR@2022

ESI学科: ENVIRONMENT/ECOLOGY;

ESI高被引阀值:17

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SCOPUS被引频次: 17

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