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作者:

Chi, Weili (Chi, Weili.) | Yang, Hong (Yang, Hong.) (学者:杨宏) | Zhang, Shude (Zhang, Shude.) | Zou, Zhiqiang (Zou, Zhiqiang.) | Wang, Xiaotong (Wang, Xiaotong.) | Wang, Shaolun (Wang, Shaolun.) | Liu, Zongyue (Liu, Zongyue.)

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摘要:

In this study, the start of partial nitrification (activated sludge)-anaerobic ammonia oxidation (immobilized fillers)-denitrification (immobilized fillers) and stable nitrogen removal in the treatment of rare earth element tailings wastewater were explored. The results showed that, at 25-30 degrees C, partial nitrification could be rapidly established by controlling the combination of average free ammonia concentration (25.4-60.2 mg/L) and dissolved oxygen concentration (0.5 mg/L). Adopting the stepwise substrate (three stages) and shortening hydraulic retention time (HRT) methods, the total nitrogen removal rate of anaerobic ammonia oxidation (anammox) immobilized fillers reached up to 0.99 kg N.(m(3).d)(-1). Adopting the C/N ratio of 4.5:1 and shorter HRT methods, the total nitrogen removal rate of denitrification immobilized fillers reached up to 1.07 kg N.(m(3).d)(-1). The activities of the anammox and denitrification immobilized fillers were increased by 8.39 and 4.46 times, respectively. At steady state operation, the average effluent ammonia nitrogen concentration was 3.01 mg/L, with an average effluent total nitrogen concentration of 5.11 mg/L, which met the requirements of the "Emission Standard for Pollutants from Rare Earth Industry" GB 26451-2011. High-throughput sequencing technology showed that the relative abundance ratios of Nitrosomonas and Nitrospira changed from 0.36:1-108.05:1. The dominant bacterial genera of the anammox immobilized fillers was Candidatus Kuenenia, and that of denitrification immobilized fillers were Pseudomonas and Thauera. This process provides a new technical approach for rare earth element tailings wastewater treatment, with high significance in engineering.

关键词:

Rare earth element tailings wastewater Anammox Immobilized fillers Microflora structure Partial nitrification

作者机构:

  • [ 1 ] [Chi, Weili]Beijing Univ Technol, Coll Architectural Engn, Key Lab Beijing Water Qual Sci & Water Environm R, Beijing 100124, Peoples R China
  • [ 2 ] [Yang, Hong]Beijing Univ Technol, Coll Architectural Engn, Key Lab Beijing Water Qual Sci & Water Environm R, Beijing 100124, Peoples R China
  • [ 3 ] [Zou, Zhiqiang]Beijing Univ Technol, Coll Architectural Engn, Key Lab Beijing Water Qual Sci & Water Environm R, Beijing 100124, Peoples R China
  • [ 4 ] [Wang, Xiaotong]Beijing Univ Technol, Coll Architectural Engn, Key Lab Beijing Water Qual Sci & Water Environm R, Beijing 100124, Peoples R China
  • [ 5 ] [Zhang, Shude]CNPC Res Inst Safety & Environm Protect Technol C, Beijing, Peoples R China
  • [ 6 ] [Wang, Shaolun]Beijing Gen Municipal Engn Design & Res Inst Co L, Beijing, Peoples R China
  • [ 7 ] [Liu, Zongyue]China Construct EcoEnvironm Grp Co LTD, Beijing, Peoples R China

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来源 :

JOURNAL OF ENVIRONMENTAL CHEMICAL ENGINEERING

ISSN: 2213-2929

年份: 2022

期: 3

卷: 10

7 . 7

JCR@2022

7 . 7 0 0

JCR@2022

JCR分区:1

中科院分区:2

被引次数:

WoS核心集被引频次: 12

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