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作者:

Chen, Dongsheng (Chen, Dongsheng.) (学者:陈东升) | Fu, Xinyi (Fu, Xinyi.) | Guo, Xiurui (Guo, Xiurui.) | Lang, Jianlei (Lang, Jianlei.) (学者:郎建垒) | Zhou, Ying (Zhou, Ying.) | Li, Yue (Li, Yue.) | Liu, Bo (Liu, Bo.) (学者:刘博) | Wang, Wenlin (Wang, Wenlin.)

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摘要:

A large amount of NOx and SO2 emitted from ships may elevate atmospheric N and S and eventually aggravate the deposition of N and S. The understanding of N and S deposition due to ship emissions is still limited, especially for China because it has a long coastline, busy shipping routes, and several large ports. To fill this gap, a comprehensive air quality model was employed in this study to quantify the contributions of ship emissions to N and S deposition on a national scale in China. Both the spatial and temporal variations of N and S deposition, as well as the major N and S species from ship traffic, were investigated. The results indicate that ship emissions contributed significantly to the deposition of N and S, especially in coastal and offshore areas, where the largest ship contribution to both N and S deposition could exceed 15 kg.ha(-1).yr(-1). For N deposition, ship emissions caused an increase in the total N deposition, not only in port areas and along shipping routes but also far inland, with evident seasonal variations. The contribution from dry N deposition was evidently larger than wet N deposition, especially over the coastal areas. S deposition, however, was generally higher along shipping routes but exhibited distinct seasonal variations. The total S deposition was dominated by dry deposition, especially over offshore areas. Ship-caused dry S deposition occurred mainly in offshore areas, while wet S deposition could be found over wider inland regions and inland waterways, although with a markedly smaller magnitude. (C) 2019 Elsevier B.V. All rights reserved.

关键词:

Ship emissions N deposition China SMOKE/WRF/CMAQ S deposition

作者机构:

  • [ 1 ] [Chen, Dongsheng]Beijing Univ Technol, Key Lab Beijing Reg Air Pollut Control, Beijing 100124, Peoples R China
  • [ 2 ] [Fu, Xinyi]Beijing Univ Technol, Key Lab Beijing Reg Air Pollut Control, Beijing 100124, Peoples R China
  • [ 3 ] [Guo, Xiurui]Beijing Univ Technol, Key Lab Beijing Reg Air Pollut Control, Beijing 100124, Peoples R China
  • [ 4 ] [Lang, Jianlei]Beijing Univ Technol, Key Lab Beijing Reg Air Pollut Control, Beijing 100124, Peoples R China
  • [ 5 ] [Zhou, Ying]Beijing Univ Technol, Key Lab Beijing Reg Air Pollut Control, Beijing 100124, Peoples R China
  • [ 6 ] [Li, Yue]Minist Transport, Transport Planning & Res Inst, Beijing 100028, Peoples R China
  • [ 7 ] [Liu, Bo]Nantong Univ, Sch Geog Sci, Nantong, Peoples R China
  • [ 8 ] [Wang, Wenlin]Minist Ecol & Environm, Nanjing Inst Environm Sci, Nanjing, Peoples R China

通讯作者信息:

  • 陈东升 刘博

    [Chen, Dongsheng]Beijing Univ Technol, Key Lab Beijing Reg Air Pollut Control, Beijing 100124, Peoples R China;;[Liu, Bo]Nantong Univ, Sch Geog Sci, Nantong, Peoples R China

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来源 :

SCIENCE OF THE TOTAL ENVIRONMENT

ISSN: 0048-9697

年份: 2020

卷: 708

9 . 8 0 0

JCR@2022

ESI学科: ENVIRONMENT/ECOLOGY;

ESI高被引阀值:138

被引次数:

WoS核心集被引频次: 23

SCOPUS被引频次: 26

ESI高被引论文在榜: 0 展开所有

万方被引频次:

中文被引频次:

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