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作者:

Han, Z. H. (Han, Z. H..) | Han, W. N. (Han, W. N..) | Liu, F. R. (Liu, F. R..) (学者:刘富荣) | Han, Z. (Han, Z..) | Yuan, Y. P. (Yuan, Y. P..) | Cheng, Z. C. (Cheng, Z. C..)

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摘要:

Studies have shown that the crystallization phase state of Ge2Sb2Te5 (GST) can be reversibly modulated by femtosecond (fs) laser multiple pulses, which have excellent applications in reconfigurable multi-level operation fields. In this study, the temporal-spatial crystalline evolution dynamics of amorphous GST film is investigated during two fs laser pulses excitation through a pump-probe shadowgraph imaging technique. A quasi-amorphous phase state, which is different from that in the initial as-deposited amorphous GST, is emerged through the first fs laser pulse excitation with a pulse energy lower than crystallization threshold. The experimental results reveal that a crystallization enhancement effect can be induced through the second pulse excitation based on this quasi-amorphous surface structure. The stimulative cluster generated in the quasi-amorphous reduces the amorphous-to-crystalline phase transition threshold for the second fs laser pulse irradiation. The spatially-resolved phase-transition threshold extension effect in a horizontal direction is proposed with the increasing pulse number to summarize the mechanism of the crystallization enhancement effect. The specific-grain-appearance (coarse grains and fine grains representing different phase transition approach) distributed area induced by single and double fs laser pulses irradiation are experimentally demonstrated corresponding to threshold extension theory.

关键词:

multiple pulse femtosecond laser phase transition evolution quasi-amorphous phase state temporal-spatial-resolved dynamics

作者机构:

  • [ 1 ] [Han, Z. H.]Beijing Univ Technol, Beijing Engn Res Ctr Appl Laser Technol, Beijing 100124, Peoples R China
  • [ 2 ] [Han, W. N.]Beijing Univ Technol, Beijing Engn Res Ctr Appl Laser Technol, Beijing 100124, Peoples R China
  • [ 3 ] [Liu, F. R.]Beijing Univ Technol, Beijing Engn Res Ctr Appl Laser Technol, Beijing 100124, Peoples R China
  • [ 4 ] [Han, Z.]Beijing Univ Technol, Beijing Engn Res Ctr Appl Laser Technol, Beijing 100124, Peoples R China
  • [ 5 ] [Yuan, Y. P.]Beijing Univ Technol, Beijing Engn Res Ctr Appl Laser Technol, Beijing 100124, Peoples R China
  • [ 6 ] [Cheng, Z. C.]Beijing Univ Technol, Beijing Engn Res Ctr Appl Laser Technol, Beijing 100124, Peoples R China
  • [ 7 ] [Han, W. N.]Beijing Inst Technol, Sch Mech Engn, Laser Micro Nano Fabricat Lab, Beijing 100081, Peoples R China

通讯作者信息:

  • [Han, W. N.]Beijing Univ Technol, Beijing Engn Res Ctr Appl Laser Technol, Beijing 100124, Peoples R China;;[Han, W. N.]Beijing Inst Technol, Sch Mech Engn, Laser Micro Nano Fabricat Lab, Beijing 100081, Peoples R China

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来源 :

NANOTECHNOLOGY

ISSN: 0957-4484

年份: 2020

期: 11

卷: 31

3 . 5 0 0

JCR@2022

ESI学科: MATERIALS SCIENCE;

ESI高被引阀值:37

JCR分区:2

被引次数:

WoS核心集被引频次: 8

SCOPUS被引频次: 12

ESI高被引论文在榜: 0 展开所有

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