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作者:

Xu, Ran (Xu, Ran.) | Zhang, Heng-De (Zhang, Heng-De.) | Yang, Xiao-Wen (Yang, Xiao-Wen.) | Cheng, Shui-Yuan (Cheng, Shui-Yuan.) (学者:程水源) | Zhang, Tian-Hang (Zhang, Tian-Hang.) | Jiang, Qi (Jiang, Qi.)

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摘要:

To study the changing of characteristics and formation mechanisms of PM2.5 in Beijing during the last two years, particulate matter concentrations, weather conditions, and air-mass trajectories were analyzed during severe pollution episodes in fall and winter 2016-2017 using routine observations and the TrajStat model. Results showed that 13 heavy pollution events, each lasting at least two days, occurred in Beijing. Of these, approximately 61.5% occurred in winter, characterized by heavier pollution concentrations and longer durations than those occurring in autumn. A low-pressure gradient, high humidity, low surface wind speed, low boundary layer, and particular terrain (i. e., being surrounded by mountains on three sides) all contributed to the high occurrence frequency of severe pollution episodes in autumn and winter. During the pollution episodes, the average ratio of PM2.5 to PM10 reached 0.86. The air-masses during the accumulation stage were mainly transported from the northwest, west, southwest, and southeast of Beijing. The southwestern and southeastern transmission paths accounted for 21.6% of the total pollution load. In addition, the WRF-CAMx model was used to quantitatively analyze the contributions of local and external sources to the concentrations of PM2.5 in Beijing during 16-22 December 2016. Based on this analysis, PM2.5 contributions notably varied with different air-masses; in the case of southern air-masses, external sources dominated the PM2.5 concentrations in Beijing and local contributions decreased rapidly; in contrast, in the case of northwestern air-masses, the opposite pattern occurred. Overall, the contribution of local sources to PM2.5 concentrations in Beijing varied from 16.5% to 69.3% during the monitored pollution episodes. © 2019, Science Press. All right reserved.

关键词:

Meteorology Boundary layers Pollution Wind

作者机构:

  • [ 1 ] [Xu, Ran]National Meteorological Center, Beijing; 100081, China
  • [ 2 ] [Zhang, Heng-De]National Meteorological Center, Beijing; 100081, China
  • [ 3 ] [Yang, Xiao-Wen]Key Laboratory of Beijing on Regional Air Pollution Control, College of Environmental and Energy Engineering, Beijing University of Technology, Beijing; 100124, China
  • [ 4 ] [Cheng, Shui-Yuan]Key Laboratory of Beijing on Regional Air Pollution Control, College of Environmental and Energy Engineering, Beijing University of Technology, Beijing; 100124, China
  • [ 5 ] [Zhang, Tian-Hang]National Meteorological Center, Beijing; 100081, China
  • [ 6 ] [Jiang, Qi]National Meteorological Center, Beijing; 100081, China

通讯作者信息:

  • [zhang, heng-de]national meteorological center, beijing; 100081, china

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来源 :

Environmental Science

ISSN: 0250-3301

年份: 2019

期: 8

卷: 40

页码: 3405-3414

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SCOPUS被引频次: 36

ESI高被引论文在榜: 0 展开所有

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