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作者:

Zheng, Jia Yu (Zheng, Jia Yu.) | He, Junda (He, Junda.) | Han, Chang Bao (Han, Chang Bao.) | Huang, Guoyu (Huang, Guoyu.) | Sun, Bei Chen (Sun, Bei Chen.) | Zhao, Wen Kang (Zhao, Wen Kang.) | Wang, Yueshuai (Wang, Yueshuai.) | Sun, Ling (Sun, Ling.) | Si, Junhui (Si, Junhui.) | Yan, Hui (Yan, Hui.)

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EI Scopus SCIE

摘要:

Improving the adsorption kinetics of metal-oxide catalysts is critical for the enhancement of catalytic perfor-mance in heterogeneous catalytic oxidation reactions. Herein, based on the biopolymer pomelo peels (PP) and metal-oxide catalyst manganese oxide (MnOx), an adsorption-enhanced catalyst (MnOx-PP) was constructed for catalytic organic dyes oxidative-degradation. MnOx-PP shows excellent methylene blue (MB) and total carbon content (TOC) removal efficiency of 99.5 % and 66.31 % respectively, and keeps the long-lasting stable dynamic degradation efficiency during 72 h based on the self-built continuous single-pass MB purification device. The chemical structure similarity and negative-charge polarity sites of the biopolymer PP improve the adsorption kinetics of organic macromolecule MB, and construct the adsorption-enhanced catalytic oxidation microenvi-ronment. Meanwhile, the adsorption-enhanced catalyst MnOx-PP obtains lower ionization potential and O2 adsorption energy to promote the continuous generation of active substance (O2*, OH*) for the further catalytic oxidation of adsorbed MB molecules. This work explored the adsorption-enhanced catalytic oxidation mecha-nism for the degradation of organic pollutants, and provided a feasible technical idea for designing adsorption-enhanced catalysts for the long-lasting efficient removal of organic dyes.

关键词:

Biopolymer pomelo peels (PP) Adsorption kinetic model Organic dyes DFT theoretical calculation Manganese oxide (MnO x )

作者机构:

  • [ 1 ] [Zheng, Jia Yu]Beijing Univ Technol, Fac Mat & Mfg, Key Lab Adv Funct Mat, Minist Educ China, Beijing 100124, Peoples R China
  • [ 2 ] [Han, Chang Bao]Beijing Univ Technol, Fac Mat & Mfg, Key Lab Adv Funct Mat, Minist Educ China, Beijing 100124, Peoples R China
  • [ 3 ] [Sun, Bei Chen]Beijing Univ Technol, Fac Mat & Mfg, Key Lab Adv Funct Mat, Minist Educ China, Beijing 100124, Peoples R China
  • [ 4 ] [Zhao, Wen Kang]Beijing Univ Technol, Fac Mat & Mfg, Key Lab Adv Funct Mat, Minist Educ China, Beijing 100124, Peoples R China
  • [ 5 ] [Wang, Yueshuai]Beijing Univ Technol, Fac Mat & Mfg, Key Lab Adv Funct Mat, Minist Educ China, Beijing 100124, Peoples R China
  • [ 6 ] [Sun, Ling]Beijing Univ Technol, Fac Mat & Mfg, Key Lab Adv Funct Mat, Minist Educ China, Beijing 100124, Peoples R China
  • [ 7 ] [Yan, Hui]Beijing Univ Technol, Fac Mat & Mfg, Key Lab Adv Funct Mat, Minist Educ China, Beijing 100124, Peoples R China
  • [ 8 ] [He, Junda]Beijing Univ Technol, Key Lab Beijing Reg Air Pollut Control, Beijing 100124, Peoples R China
  • [ 9 ] [Huang, Guoyu]Beijing Univ Technol, Fac Mat & Mfg, Beijing Key Lab Microstruct & Properties Solids, Beijing 100124, Peoples R China
  • [ 10 ] [Si, Junhui]Fujian Univ Technol, Coll Mat Sci & Engn, Fuzhou 350118, Fujian, Peoples R China

通讯作者信息:

  • [Han, Chang Bao]Beijing Univ Technol, Fac Mat & Mfg, Key Lab Adv Funct Mat, Minist Educ China, Beijing 100124, Peoples R China;;[Si, Junhui]Fujian Univ Technol, Coll Mat Sci & Engn, Fuzhou 350118, Fujian, Peoples R China;;

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来源 :

INTERNATIONAL JOURNAL OF BIOLOGICAL MACROMOLECULES

ISSN: 0141-8130

年份: 2023

卷: 237

8 . 2 0 0

JCR@2022

ESI学科: BIOLOGY & BIOCHEMISTRY;

ESI高被引阀值:16

被引次数:

WoS核心集被引频次:

SCOPUS被引频次: 11

ESI高被引论文在榜: 0 展开所有

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中文被引频次:

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