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Author:

Sun, Yajie (Sun, Yajie.) | Pei, Xinya (Pei, Xinya.) | Wang, Bo (Wang, Bo.) | Ng, Yun Hau (Ng, Yun Hau.) | Zhu, Ruixue (Zhu, Ruixue.) | Zhang, Qichao (Zhang, Qichao.) | Deng, Jiguang (Deng, Jiguang.) | Liu, Yuxi (Liu, Yuxi.) | Jing, Lin (Jing, Lin.) | Dai, Hongxing (Dai, Hongxing.)

Indexed by:

EI Scopus SCIE

Abstract:

Red phosphorus (RP) has been demonstrated for photocatalytic hydrogen evolution (PHE) in recent years. Realistically, P vacancy (VP) defects are present in RP. The constructive or detrimental influences of such defects on the photocatalytic activity of RP should be revealed as the understanding shall provide a platform for further improvement. Herein, we for the first time establish a comprehensive understanding of the crucial relationships between the intrinsic VP defects and the charge dynamics together with the photocatalytic performance in RP. Two main findings are achieved: i) VP-induced deep charge trapping effect is revealed to lead to a severe loss of active electrons during the H+ reduction reaction, resulting in the inferior PHE performance of RP. ii) O doping in the VP sites is demonstrated to be an effective strategy for eliminating the detrimental VP defect states, leading to a long-lived free electron lifetime in RP for enhanced PHE performance. The point defect engineering of RP applied in this study paves a promising way in tuning the physicochemical properties of RP and other elemental -based materials for various applications.

Keyword:

Phosphorus vacancies Hydrogen evolution Red phosphorus Elemental photocatalyst Defect engineering

Author Community:

  • [ 1 ] [Sun, Yajie]Beijing Univ Technol, Beijing Key Lab Green Catalysis & Separat, Beijing 100124, Peoples R China
  • [ 2 ] [Pei, Xinya]Beijing Univ Technol, Beijing Key Lab Green Catalysis & Separat, Beijing 100124, Peoples R China
  • [ 3 ] [Zhang, Qichao]Beijing Univ Technol, Beijing Key Lab Green Catalysis & Separat, Beijing 100124, Peoples R China
  • [ 4 ] [Deng, Jiguang]Beijing Univ Technol, Beijing Key Lab Green Catalysis & Separat, Beijing 100124, Peoples R China
  • [ 5 ] [Liu, Yuxi]Beijing Univ Technol, Beijing Key Lab Green Catalysis & Separat, Beijing 100124, Peoples R China
  • [ 6 ] [Jing, Lin]Beijing Univ Technol, Beijing Key Lab Green Catalysis & Separat, Beijing 100124, Peoples R China
  • [ 7 ] [Dai, Hongxing]Beijing Univ Technol, Beijing Key Lab Green Catalysis & Separat, Beijing 100124, Peoples R China
  • [ 8 ] [Sun, Yajie]Beijing Univ Technol, Fac Environm & Life, Beijing 100124, Peoples R China
  • [ 9 ] [Pei, Xinya]Beijing Univ Technol, Fac Environm & Life, Beijing 100124, Peoples R China
  • [ 10 ] [Zhang, Qichao]Beijing Univ Technol, Fac Environm & Life, Beijing 100124, Peoples R China
  • [ 11 ] [Deng, Jiguang]Beijing Univ Technol, Fac Environm & Life, Beijing 100124, Peoples R China
  • [ 12 ] [Liu, Yuxi]Beijing Univ Technol, Fac Environm & Life, Beijing 100124, Peoples R China
  • [ 13 ] [Jing, Lin]Beijing Univ Technol, Fac Environm & Life, Beijing 100124, Peoples R China
  • [ 14 ] [Dai, Hongxing]Beijing Univ Technol, Fac Environm & Life, Beijing 100124, Peoples R China
  • [ 15 ] [Wang, Bo]Beijing Univ Technol, Engn Res Ctr Beijing, Natl Engn Lab Adv Municipal Wastewater Treatment &, Beijing, Peoples R China
  • [ 16 ] [Ng, Yun Hau]City Univ Hong Kong, Sch Energy & Environm, Kowloon, Tat Chee Ave, Hong Kong, Peoples R China
  • [ 17 ] [Ng, Yun Hau]City Univ Hong Kong, Shenzhen Res Inst, Shenzhen Hitech Ind Pk, Shenzhen 518057, Peoples R China
  • [ 18 ] [Zhu, Ruixue]ShanghaiTech Univ, Ctr Transformat Sci, Shanghai 201210, Peoples R China

Reprint Author's Address:

  • [Jing, Lin]Beijing Univ Technol, Beijing Key Lab Green Catalysis & Separat, Beijing 100124, Peoples R China;;[Jing, Lin]Beijing Univ Technol, Fac Environm & Life, Beijing 100124, Peoples R China;;

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Source :

CHEMICAL ENGINEERING JOURNAL

ISSN: 1385-8947

Year: 2023

Volume: 463

1 5 . 1 0 0

JCR@2022

ESI Discipline: ENGINEERING;

ESI HC Threshold:19

Cited Count:

WoS CC Cited Count:

SCOPUS Cited Count: 23

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 3

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