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Abstract:
Monoclinic beta-Ga2O3 microbelts were successfully fabricated using a one-step optical vapor supersaturated precipitation method, which exhibited advantages including a free-standing substrate, prefect surface, and low cost. The as-grown microbelts possessed a well-defined geometry and perfect crystallinity. The dimensions of individual b-Ga2O3 microbelts were a width of similar to 50 mu m, length of similar to 5 mm, and thickness of similar to 3 mu m. The SEM, XRD, HRTEM, XPS, and Raman spectra demonstrated the high single-crystalline structure of b-Ga2O3 microbelts. Twelve frequency modes were activated in Raman spectra. The optical band gap of the beta-Ga2O3 microbelt was calculated to be similar to 4.45 eV. Upon 266 nm excitation, 2 strong UV emissions occurred in photoluminescence spectra through the radiative recombination of self-trapped excitons, and the blue emission band was attributed to the presence of donor-acceptor-pair transition. The individual b-Ga2O3 microbelt was employed as metal-semiconductor-metal deep-ultraviolet photodetector, which exhibits the photoresponse under 254 nm. This work provides a simple and economical route to fabricate high-quality beta-Ga2O3 single-crystal microbelts, which should be a potential synthetic strategy for ultra-wide bandgap semiconductor materials.
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CRYSTALS
Year: 2023
Issue: 5
Volume: 13
2 . 7 0 0
JCR@2022
ESI Discipline: MATERIALS SCIENCE;
ESI HC Threshold:26
Cited Count:
WoS CC Cited Count: 6
SCOPUS Cited Count: 6
ESI Highly Cited Papers on the List: 0 Unfold All
WanFang Cited Count:
Chinese Cited Count:
30 Days PV: 2
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