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Author:

Pan, Yongman (Pan, Yongman.) | Wang, Qiang (Wang, Qiang.) | Yan, Yinzhou (Yan, Yinzhou.) | Yang, Lixue (Yang, Lixue.) | Wan, Lingyu (Wan, Lingyu.) | Yao, Rongcheng (Yao, Rongcheng.) | Jiang, Yijian (Jiang, Yijian.)

Indexed by:

Scopus SCIE

Abstract:

Monoclinic beta-Ga2O3 microbelts were successfully fabricated using a one-step optical vapor supersaturated precipitation method, which exhibited advantages including a free-standing substrate, prefect surface, and low cost. The as-grown microbelts possessed a well-defined geometry and perfect crystallinity. The dimensions of individual b-Ga2O3 microbelts were a width of similar to 50 mu m, length of similar to 5 mm, and thickness of similar to 3 mu m. The SEM, XRD, HRTEM, XPS, and Raman spectra demonstrated the high single-crystalline structure of b-Ga2O3 microbelts. Twelve frequency modes were activated in Raman spectra. The optical band gap of the beta-Ga2O3 microbelt was calculated to be similar to 4.45 eV. Upon 266 nm excitation, 2 strong UV emissions occurred in photoluminescence spectra through the radiative recombination of self-trapped excitons, and the blue emission band was attributed to the presence of donor-acceptor-pair transition. The individual b-Ga2O3 microbelt was employed as metal-semiconductor-metal deep-ultraviolet photodetector, which exhibits the photoresponse under 254 nm. This work provides a simple and economical route to fabricate high-quality beta-Ga2O3 single-crystal microbelts, which should be a potential synthetic strategy for ultra-wide bandgap semiconductor materials.

Keyword:

microbelts photoconductivity beta-Ga2O3 photoluminescence OVSP

Author Community:

  • [ 1 ] [Pan, Yongman]Beijing Univ Technol, Inst Laser Engn, Fac Mat & Mfg, Beijing 100124, Peoples R China
  • [ 2 ] [Yan, Yinzhou]Beijing Univ Technol, Inst Laser Engn, Fac Mat & Mfg, Beijing 100124, Peoples R China
  • [ 3 ] [Jiang, Yijian]Beijing Univ Technol, Inst Laser Engn, Fac Mat & Mfg, Beijing 100124, Peoples R China
  • [ 4 ] [Pan, Yongman]Beijing Univ Technol, Inst Matter Sci, Beijing 100124, Peoples R China
  • [ 5 ] [Yan, Yinzhou]Beijing Univ Technol, Inst Matter Sci, Beijing 100124, Peoples R China
  • [ 6 ] [Jiang, Yijian]Beijing Univ Technol, Inst Matter Sci, Beijing 100124, Peoples R China
  • [ 7 ] [Pan, Yongman]Beijing Univ Technol, Key Lab Transscale Laser Mfg Technol, Minist Educ, Beijing 100124, Peoples R China
  • [ 8 ] [Yan, Yinzhou]Beijing Univ Technol, Key Lab Transscale Laser Mfg Technol, Minist Educ, Beijing 100124, Peoples R China
  • [ 9 ] [Jiang, Yijian]Beijing Univ Technol, Key Lab Transscale Laser Mfg Technol, Minist Educ, Beijing 100124, Peoples R China
  • [ 10 ] [Wang, Qiang]Beijing Inst Petrochem Technol, Coll New Mat & Chem Engn, Beijing 102617, Peoples R China
  • [ 11 ] [Yang, Lixue]Beijing Inst Graph Commun, Sch Printing & Packing Engineer, Beijing 102627, Peoples R China
  • [ 12 ] [Wan, Lingyu]Guangxi Univ, Sch Phys Sci & Technol, Nanning 530004, Peoples R China
  • [ 13 ] [Yao, Rongcheng]Guangxi Univ, Sch Phys Sci & Technol, Nanning 530004, Peoples R China

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Source :

CRYSTALS

Year: 2023

Issue: 5

Volume: 13

2 . 7 0 0

JCR@2022

ESI Discipline: MATERIALS SCIENCE;

ESI HC Threshold:26

Cited Count:

WoS CC Cited Count: 6

SCOPUS Cited Count: 6

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 2

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