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Author:

Li, Yang (Li, Yang.) | Ding, Peipei (Ding, Peipei.) | Gu, Yuzhe (Gu, Yuzhe.) | Qian, Sheng (Qian, Sheng.) | Pang, Yuncong (Pang, Yuncong.) | Wang, Lele (Wang, Lele.) | Feng, Jiayang (Feng, Jiayang.) | Liu, Baoguang (Liu, Baoguang.) | Wan, Qi (Wan, Qi.) | Li, Ping (Li, Ping.) | Liu, Zhiwei (Liu, Zhiwei.)

Indexed by:

EI Scopus SCIE

Abstract:

In the green energy and carbon-neutral technology, electrochemical energy storage devices have received continuously increasing attention recently. However, due to the unavoidable volume expansion/shrinkage of key materials or irreversible mechanical damages during application, the stability of energy storage and delivery as well as the lifetime of these devices are severely shortened, leading to serious performance degradation or even safety issues. Therefore, the utilization of self-healable gels into electrochemical energy storage devices, such as electrodes, binders, and electrolytes, is proven as an effective method to realize long-term stable operation of these devices via the self-repairing of mechanical and electrochemical characteristics. Herein, this review first summarizes the feature and fabrication of different gels, paying special attention to hydrogels, organohydrogels, and ionogels. Then, basic concepts and figure of merit of self-healable gels are analyzed with a detailed discussion at the healing mechanisms, from reversible dynamic bonds to physical molecular diffusion, and to external healing trigger. Then we introduce all the important parts of electrochemical energy storage devices, which could be replaced by healable gels to enhance the durability, including electrodes, binders, and electrolytes. Finally, the critical challenges and future perspectives regarding the future development of healable gels based high-performance electrochemical energy storage devices or electronics are provided.

Keyword:

gel electrolytes self-healable gels healing mechanisms electrodes binders

Author Community:

  • [ 1 ] [Li, Yang]Nanjing Univ Posts & Telecommun NJUPT, Coll Elect & Opt Engn, Nanjing 210023, Peoples R China
  • [ 2 ] [Gu, Yuzhe]Nanjing Univ Posts & Telecommun NJUPT, Coll Elect & Opt Engn, Nanjing 210023, Peoples R China
  • [ 3 ] [Wang, Lele]Nanjing Univ Posts & Telecommun NJUPT, Coll Elect & Opt Engn, Nanjing 210023, Peoples R China
  • [ 4 ] [Feng, Jiayang]Nanjing Univ Posts & Telecommun NJUPT, Coll Elect & Opt Engn, Nanjing 210023, Peoples R China
  • [ 5 ] [Liu, Baoguang]Nanjing Univ Posts & Telecommun NJUPT, Coll Elect & Opt Engn, Nanjing 210023, Peoples R China
  • [ 6 ] [Li, Yang]Nanjing Univ Posts & Telecommun NJUPT, Coll Flexible Elect Future Technol, Nanjing 210023, Peoples R China
  • [ 7 ] [Gu, Yuzhe]Nanjing Univ Posts & Telecommun NJUPT, Coll Flexible Elect Future Technol, Nanjing 210023, Peoples R China
  • [ 8 ] [Wang, Lele]Nanjing Univ Posts & Telecommun NJUPT, Coll Flexible Elect Future Technol, Nanjing 210023, Peoples R China
  • [ 9 ] [Feng, Jiayang]Nanjing Univ Posts & Telecommun NJUPT, Coll Flexible Elect Future Technol, Nanjing 210023, Peoples R China
  • [ 10 ] [Liu, Baoguang]Nanjing Univ Posts & Telecommun NJUPT, Coll Flexible Elect Future Technol, Nanjing 210023, Peoples R China
  • [ 11 ] [Li, Yang]Nanjing Univ Posts & Telecommun NJUPT, Inst Adv Mat IAM, State Key Lab Organ Elect & Informat Displays, Nanjing 210023, Peoples R China
  • [ 12 ] [Qian, Sheng]Nanjing Univ Posts & Telecommun NJUPT, Inst Adv Mat IAM, State Key Lab Organ Elect & Informat Displays, Nanjing 210023, Peoples R China
  • [ 13 ] [Pang, Yuncong]Nanjing Univ Posts & Telecommun NJUPT, Inst Adv Mat IAM, State Key Lab Organ Elect & Informat Displays, Nanjing 210023, Peoples R China
  • [ 14 ] [Li, Yang]Nanjing Univ Posts & Telecommun NJUPT, Inst Adv Mat IAM, Jiangsu Key Lab Biosensors, Nanjing 210023, Peoples R China
  • [ 15 ] [Qian, Sheng]Nanjing Univ Posts & Telecommun NJUPT, Inst Adv Mat IAM, Jiangsu Key Lab Biosensors, Nanjing 210023, Peoples R China
  • [ 16 ] [Pang, Yuncong]Nanjing Univ Posts & Telecommun NJUPT, Inst Adv Mat IAM, Jiangsu Key Lab Biosensors, Nanjing 210023, Peoples R China
  • [ 17 ] [Ding, Peipei]Beijing Univ Technol, Coll Mat Sci & Engn, Beijing 100124, Peoples R China
  • [ 18 ] [Wan, Qi]Univ Sci & Technol Beijing, Inst Adv Mat & Technol, Beijing Adv Innovat Ctr Mat Genome Engn, Beijing 100083, Peoples R China
  • [ 19 ] [Li, Ping]Univ Sci & Technol Beijing, Inst Adv Mat & Technol, Beijing Adv Innovat Ctr Mat Genome Engn, Beijing 100083, Peoples R China
  • [ 20 ] [Liu, Zhiwei]Singapore Univ Technol & Design, Pillar Engn Prod Dev, Singapore 487372, Singapore
  • [ 21 ] [Liu, Zhiwei]Univ Sci & Technol Beijing, Sch Energy & Environm Engn, Beijing 100083, Peoples R China

Reprint Author's Address:

  • [Li, Yang]Nanjing Univ Posts & Telecommun NJUPT, Coll Elect & Opt Engn, Nanjing 210023, Peoples R China;;[Li, Yang]Nanjing Univ Posts & Telecommun NJUPT, Coll Flexible Elect Future Technol, Nanjing 210023, Peoples R China;;[Li, Yang]Nanjing Univ Posts & Telecommun NJUPT, Inst Adv Mat IAM, State Key Lab Organ Elect & Informat Displays, Nanjing 210023, Peoples R China;;[Li, Yang]Nanjing Univ Posts & Telecommun NJUPT, Inst Adv Mat IAM, Jiangsu Key Lab Biosensors, Nanjing 210023, Peoples R China;;[Liu, Zhiwei]Singapore Univ Technol & Design, Pillar Engn Prod Dev, Singapore 487372, Singapore;;[Liu, Zhiwei]Univ Sci & Technol Beijing, Sch Energy & Environm Engn, Beijing 100083, Peoples R China;;

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Source :

NANO RESEARCH

ISSN: 1998-0124

Year: 2023

Issue: 4

Volume: 17

Page: 3302-3323

9 . 9 0 0

JCR@2022

ESI Discipline: PHYSICS;

ESI HC Threshold:17

Cited Count:

WoS CC Cited Count:

SCOPUS Cited Count: 10

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 1

Affiliated Colleges:

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