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作者:

Fan, Xiao-Chen (Fan, Xiao-Chen.) | Lang, Jian-Lei (Lang, Jian-Lei.) (学者:郎建垒) | Cheng, Shui-Yuan (Cheng, Shui-Yuan.) (学者:程水源) | Wang, Xiao-Qi (Wang, Xiao-Qi.) | Lü, Zhe (Lü, Zhe.)

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摘要:

Atmospheric particulate matter is the primary pollutant affecting the ambient air quality in most Chinese cities. In recent years, with the progress of monitoring technology and improvement in sampling equipment, the relevant research objects gradually shift from larger particle sizes (PM10 and PM2.5) to smaller particle size (PM1). The carbonaceous component is an important part of atmospheric particulate matter. Taking Beijing as the research area, sampling for PM2.5 and PM1 was conducted in July and October of 2016, and January and April of 2017 as representative months of four seasons. Mass concentrations and seasonal variation characteristics for PM2.5 and PM1 were analyzed. The two-layer, nested, meteorology-air quality coupling model system (WRF-CMAQ) was used to model air circulation during the sampling period and thus analyze the source contributions for PM2.5 and PM1. The factor analysis method was also used to analyze the source apportionment of carbonaceous components. The results are as followed: the mass concentrations of PM2.5 and PM1 showed an increasing trend by spring, summer, autumn and winter. PM1 was the main part of PM2.5, and with the increasing frequency of haze in autumn and winter, the mass concentration ratio of PM1/PM2.5 became significantly higher. The authors contend that secondary pollution exists in Beijing's atmosphere, and SOC is more likely to accumulate in smaller particle size. Widespread coal combustion, vehicle emission, residential emission source and biomass combustion emissions are the major contributors to atmospheric particulates, while gasoline engine exhaust, diesel vehicle exhaust, biomass combustion and coal combustion emission are the main source of carbonaceous components in PM2.5 and PM1 in Beijing. © 2018, Science Press. All right reserved.

关键词:

Air quality Coal combustion Particle size Particle size analysis Particles (particulate matter)

作者机构:

  • [ 1 ] [Fan, Xiao-Chen]Key Laboratory of Beijing on Regional Air Pollution Control, College of Environmental and Energy Engineering, Beijing University of Technology, Beijing; 100124, China
  • [ 2 ] [Lang, Jian-Lei]Key Laboratory of Beijing on Regional Air Pollution Control, College of Environmental and Energy Engineering, Beijing University of Technology, Beijing; 100124, China
  • [ 3 ] [Cheng, Shui-Yuan]Key Laboratory of Beijing on Regional Air Pollution Control, College of Environmental and Energy Engineering, Beijing University of Technology, Beijing; 100124, China
  • [ 4 ] [Wang, Xiao-Qi]Key Laboratory of Beijing on Regional Air Pollution Control, College of Environmental and Energy Engineering, Beijing University of Technology, Beijing; 100124, China
  • [ 5 ] [Lü, Zhe]Key Laboratory of Beijing on Regional Air Pollution Control, College of Environmental and Energy Engineering, Beijing University of Technology, Beijing; 100124, China

通讯作者信息:

  • 程水源

    [cheng, shui-yuan]key laboratory of beijing on regional air pollution control, college of environmental and energy engineering, beijing university of technology, beijing; 100124, china

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来源 :

Environmental Science

ISSN: 0250-3301

年份: 2018

期: 10

卷: 39

页码: 4430-4438

被引次数:

WoS核心集被引频次: 0

SCOPUS被引频次: 15

ESI高被引论文在榜: 0 展开所有

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