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作者:

Yang Huang-Gen (Yang Huang-Gen.) | Chen Yuan (Chen Yuan.) | Wang Zhi-Wei (Wang Zhi-Wei.) | Yang Jia-Tian (Yang Jia-Tian.) | Zhu Li-Gang (Zhu Li-Gang.) | Qin Li-Qin (Qin Li-Qin.) | Dai Hong-Xing (Dai Hong-Xing.) (学者:戴洪兴)

收录:

SCIE CSCD

摘要:

Porous nanosheet-aggregated persimmon-like bismuth oxybromide (BiOBr) were successfully prepared for the first time using polyvinyl pyrrolidone (PVP)-assistctd solvothermal strategy with bismuth nitrate and cetyltrimethyl ammonium bromide (CTAB) as Bi and Br sources. Physicochemical properties of the hierarchical microstructure BiOBr materials were characterized by means of numerous analytical techniques, and their pholocatalytic activities were evaluated for the removal of methylene blue (MB) under visible-light illumination. It is found that the solvothermal time and PVP addition had a significant influence on the particle morphology and crystallinity of the product. The porous sheet-aggregated persimmon-like BiOBr sample could be obtained after solvothermal treatment at 120 degrees C, for 12 h in the presence of 0.7 g PVP. The porous persimmon-like BiOBr sample with a surface area of 4 m(2).g(-1) and a bandgap energy of 2.64 eV possessed good optical absorption property in visible-light regions and showed excellent visible-light-driven photocatalytic activity and stability for MB degradation. It is concluded that the high visible-light-driven catalytic performance of the porous sheet-aggregated persimmon-like BiOBr sample is associated with its high surface area, porous structure, and low bandgap energy as well as the unique particle morphology.

关键词:

hierarchical microstructure organic dye degradation persimmon-like BiOBr solvothermal synthesis visible-light-driven photocatalysis

作者机构:

  • [ 1 ] [Yang Huang-Gen]Yulin Normal Univ, Coll Chem & Food Sci, Guangxi Key Lab Agr Resources Chem & Biotechnol, Yulin 537000, Guangxi, Peoples R China
  • [ 2 ] [Chen Yuan]Yulin Normal Univ, Coll Chem & Food Sci, Guangxi Key Lab Agr Resources Chem & Biotechnol, Yulin 537000, Guangxi, Peoples R China
  • [ 3 ] [Yang Jia-Tian]Yulin Normal Univ, Coll Chem & Food Sci, Guangxi Key Lab Agr Resources Chem & Biotechnol, Yulin 537000, Guangxi, Peoples R China
  • [ 4 ] [Zhu Li-Gang]Yulin Normal Univ, Coll Chem & Food Sci, Guangxi Key Lab Agr Resources Chem & Biotechnol, Yulin 537000, Guangxi, Peoples R China
  • [ 5 ] [Qin Li-Qin]Yulin Normal Univ, Coll Chem & Food Sci, Guangxi Key Lab Agr Resources Chem & Biotechnol, Yulin 537000, Guangxi, Peoples R China
  • [ 6 ] [Wang Zhi-Wei]Beijing Univ Technol, Coll Environm & Energy Engn, Beijing Key Lab Green Catalysis & Separat,Educ Mi, Key Lab Beijing Reg Air Pollut Control,Key Lab Ad, Beijing 100124, Peoples R China
  • [ 7 ] [Dai Hong-Xing]Beijing Univ Technol, Coll Environm & Energy Engn, Beijing Key Lab Green Catalysis & Separat,Educ Mi, Key Lab Beijing Reg Air Pollut Control,Key Lab Ad, Beijing 100124, Peoples R China
  • [ 8 ] [Wang Zhi-Wei]Beijing Univ Technol, Coll Environm & Energy Engn, Lab Catalysis Chem & Nanosci, Dept Chem & Chem Engn, Beijing 100124, Peoples R China
  • [ 9 ] [Dai Hong-Xing]Beijing Univ Technol, Coll Environm & Energy Engn, Lab Catalysis Chem & Nanosci, Dept Chem & Chem Engn, Beijing 100124, Peoples R China

通讯作者信息:

  • 戴洪兴

    [Chen Yuan]Yulin Normal Univ, Coll Chem & Food Sci, Guangxi Key Lab Agr Resources Chem & Biotechnol, Yulin 537000, Guangxi, Peoples R China;;[Dai Hong-Xing]Beijing Univ Technol, Coll Environm & Energy Engn, Beijing Key Lab Green Catalysis & Separat,Educ Mi, Key Lab Beijing Reg Air Pollut Control,Key Lab Ad, Beijing 100124, Peoples R China;;[Dai Hong-Xing]Beijing Univ Technol, Coll Environm & Energy Engn, Lab Catalysis Chem & Nanosci, Dept Chem & Chem Engn, Beijing 100124, Peoples R China

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来源 :

CHINESE JOURNAL OF INORGANIC CHEMISTRY

ISSN: 1001-4861

年份: 2020

期: 2

卷: 36

页码: 333-344

0 . 7 0 0

JCR@2022

ESI学科: CHEMISTRY;

ESI高被引阀值:33

JCR分区:4

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