Interface science in polymer-based composite solid electrolytes in lithium metal batteries - 文章详情页

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Solid-state　lithium　metal　batteries　(SSLMBs)　have　attracted　considerable　attention　as　one　of　the　most　promising　energy　storage　systems　owing　to　their　high　safety　and　energy　density.　Solid　electrolytes,　particularly　polymer-based　composite　solid　electrolytes　(CSEs),　are　considered　promising　electrolyte　candidates　for　SSLMBs.　However,　their　wide　application　is　inhibited　by　various　electrochemical　issues,　such　as　low　ionic　conductivity,　the　growth　of　lithium　dendrites,　and　poor　cycling　stability,　which　are　related　to　interface　issues　within　SSLMBs.　In　this　review,　the　parameters　related　to　various　interfaces　in　the　CSE　of　SSLMBs,　including　the　interfaces　between　the　polymer　matrix　and　inorganic　fillers,　between　the　CSEs　and　the　cathode,　and　between　the　CSEs　and　the　lithium　metal　anode,　are　examined.　Relevant　issues　and　corresponding　remediation　strategies　are　proposed.　Finally,　future　perspectives　based　on　interfacial　engineering　and　the　characterization　of　polymer/inorganic　filler　interactions　are　proposed　for　building　high-performance　CSEs　for　use　in　SSLMBs.　©　2022　The　Authors.　SusMat　published　by　Sichuan　University　and　John　Wiley　&　Sons　Australia,　Ltd.

关键词：

Fillers Electrodes Lithium Filled polymers Solid-State Batteries Interface states Lithium batteries Solid electrolytes

作者机构：

[ 1 ] [Wu, Lingqiao]Faculty of Materials and Manufacturing, Institute of Advanced Battery Materials and Devices, Beijing University of Technology, Beijing, China
[ 2 ] [Wu, Lingqiao]Key Laboratory of Advanced Functional Materials, Ministry of Education, Beijing University of Technology, Beijing, China
[ 3 ] [Wang, Yongtao]Faculty of Materials and Manufacturing, Institute of Advanced Battery Materials and Devices, Beijing University of Technology, Beijing, China
[ 4 ] [Wang, Yongtao]Key Laboratory of Advanced Functional Materials, Ministry of Education, Beijing University of Technology, Beijing, China
[ 5 ] [Guo, Xianwei]Faculty of Materials and Manufacturing, Institute of Advanced Battery Materials and Devices, Beijing University of Technology, Beijing, China
[ 6 ] [Guo, Xianwei]Key Laboratory of Advanced Functional Materials, Ministry of Education, Beijing University of Technology, Beijing, China
[ 7 ] [Ding, Peipei]Faculty of Materials and Manufacturing, Institute of Advanced Battery Materials and Devices, Beijing University of Technology, Beijing, China
[ 8 ] [Ding, Peipei]Key Laboratory of Advanced Functional Materials, Ministry of Education, Beijing University of Technology, Beijing, China
[ 9 ] [Lin, Zhiyuan]Faculty of Materials and Manufacturing, Institute of Advanced Battery Materials and Devices, Beijing University of Technology, Beijing, China
[ 10 ] [Lin, Zhiyuan]Key Laboratory of Advanced Functional Materials, Ministry of Education, Beijing University of Technology, Beijing, China
[ 11 ] [Yu, Haijun]Faculty of Materials and Manufacturing, Institute of Advanced Battery Materials and Devices, Beijing University of Technology, Beijing, China
[ 12 ] [Yu, Haijun]Key Laboratory of Advanced Functional Materials, Ministry of Education, Beijing University of Technology, Beijing, China

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