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作者:

Cai, Yuanyuan (Cai, Yuanyuan.) | Nie, Zuoren (Nie, Zuoren.) | Ma, Liwen (Ma, Liwen.) | Xi, Xiaoli (Xi, Xiaoli.) (学者:席晓丽)

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EI Scopus SCIE

摘要:

As metal additive manufacturing (MAM) technology is booming in the aerospace sector, alternatives to the traditional production methods of metals such as mining, processing, and refining with severe emissions are urgently needed. This study proposed a closed-loop route for efficient recovery of molybdenum (Mo) and valueadded reuse of tungsten (W) from Cr-Co-Ni-Mo-W alloy waste in MAM. The results showed that the leaching efficiency of Mo and W reached 99.3% and 99.9%, respectively, using the dual chemical-physical means of mixed-alkali roasting and leaching by microwave heating, while the discharge of waste liquor containing Cr6+ was reduced. Leaching kinetic studies revealed that the metal leaching process was controlled by chemical reaction mechanism. Moreover, the 10%N1923 (primary amine)-5%TRPO (tri-alkyl phosphine oxide)-kerosene extraction system exhibited a synergistic extraction effect on Mo and W. After purification, Mo was recovered as Mo powder for MAM. Simultaneously, the recovered product of W, MnWO4, was applied as a photocatalytic material with excellent degradation of methylene blue dye. Ultimately, the proposed method obtained recovery efficiencies of 98.4% and 99.3% for Mo and W, respectively, achieving efficient and environmentally-friendly reuse of these key metals.

关键词:

Molybdenum Extraction Tungsten Metal additive manufacturing Alloy waste

作者机构:

  • [ 1 ] [Cai, Yuanyuan]Beijing Univ Technol, Fac Mat & Mfg, Collaborat Innovat Ctr Capital Resource Recycling, Beijing 100124, Peoples R China
  • [ 2 ] [Nie, Zuoren]Beijing Univ Technol, Fac Mat & Mfg, Collaborat Innovat Ctr Capital Resource Recycling, Beijing 100124, Peoples R China
  • [ 3 ] [Ma, Liwen]Beijing Univ Technol, Fac Mat & Mfg, Collaborat Innovat Ctr Capital Resource Recycling, Beijing 100124, Peoples R China
  • [ 4 ] [Xi, Xiaoli]Beijing Univ Technol, Fac Mat & Mfg, Collaborat Innovat Ctr Capital Resource Recycling, Beijing 100124, Peoples R China
  • [ 5 ] [Nie, Zuoren]Beijing Univ Technol, Key Lab Adv Funct Mat, Minist Educ, Beijing 100124, Peoples R China
  • [ 6 ] [Xi, Xiaoli]Beijing Univ Technol, Key Lab Adv Funct Mat, Minist Educ, Beijing 100124, Peoples R China
  • [ 7 ] [Nie, Zuoren]Beijing Univ Technol, Natl Engn Lab Ind Bigdata Applicat Technol, Beijing 100124, Peoples R China
  • [ 8 ] [Ma, Liwen]Beijing Univ Technol, Natl Engn Lab Ind Bigdata Applicat Technol, Beijing 100124, Peoples R China
  • [ 9 ] [Xi, Xiaoli]Beijing Univ Technol, Fac Mat & Mfg, 100 Pingleyuan, Beijing 100124, Peoples R China

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来源 :

JOURNAL OF ENVIRONMENTAL MANAGEMENT

ISSN: 0301-4797

年份: 2023

卷: 348

8 . 7 0 0

JCR@2022

被引次数:

WoS核心集被引频次: 6

SCOPUS被引频次: 6

ESI高被引论文在榜: 0 展开所有

万方被引频次:

中文被引频次:

近30日浏览量: 3

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