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作者:

Li, Yi Tong (Li, Yi Tong.) | Guo, Hang (Guo, Hang.) | Ye, Fang (Ye, Fang.) | Chen, Hao (Chen, Hao.)

收录:

EI Scopus SCIE

摘要:

Platinum loading and electrolyte content affect the surface area of electrochemical reaction and proton conductivity, respectively, and protons and oxygen are not uniformly distributed in the catalyst layer. Therefore, platinum loading and electrolyte content can be set to be simultaneous non-uniform distributions to further enhance the species utilization and cell performance. In this study, a non-isothermal, two-dimensional, twophase fuel cell model is set up and coupled with the catalyst layer agglomerate model. The electrolyte content and platinum loading uneven distributions influence on products and reactants transmission and electrical property is explored. Results indicate that electrolyte volume fraction and platinum loading coinstantaneous graded distribution is more helpful in the species transfer and electrical property improvement. The maximum power density of coinstantaneous graded distribution of platinum content and electrolyte loading along the channel direction is increased by 3.40% compared with the uniform distribution, and is 2.94% higher than the superposition of the maximum power density when the graded distributions of electrolyte volume fraction and platinum loading are separately set. Moreover, the platinum content and electrolyte content gradient distributions do not make liquid water saturation present an evident segment variation along the channel direction, while the opposite is true for oxygen concentration.

关键词:

Mass transfer Catalyst layer composition Uneven distribution Proton exchange membrane fuel cell Performance

作者机构:

  • [ 1 ] [Li, Yi Tong]Beijing Univ Technol, MOE Key Lab Enhanced Heat Transfer & Energy Conser, Beijing Key Lab Heat Transfer & Energy Convers, Beijing 100124, Peoples R China
  • [ 2 ] [Guo, Hang]Beijing Univ Technol, MOE Key Lab Enhanced Heat Transfer & Energy Conser, Beijing Key Lab Heat Transfer & Energy Convers, Beijing 100124, Peoples R China
  • [ 3 ] [Ye, Fang]Beijing Univ Technol, MOE Key Lab Enhanced Heat Transfer & Energy Conser, Beijing Key Lab Heat Transfer & Energy Convers, Beijing 100124, Peoples R China
  • [ 4 ] [Chen, Hao]Beijing Univ Technol, MOE Key Lab Enhanced Heat Transfer & Energy Conser, Beijing Key Lab Heat Transfer & Energy Convers, Beijing 100124, Peoples R China

通讯作者信息:

  • [Guo, Hang]Beijing Univ Technol, MOE Key Lab Enhanced Heat Transfer & Energy Conser, Beijing Key Lab Heat Transfer & Energy Convers, Beijing 100124, Peoples R China;;

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来源 :

INTERNATIONAL COMMUNICATIONS IN HEAT AND MASS TRANSFER

ISSN: 0735-1933

年份: 2023

卷: 150

7 . 0 0 0

JCR@2022

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WoS核心集被引频次: 1

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ESI高被引论文在榜: 0 展开所有

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