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作者:

Gan, Yanling (Gan, Yanling.) | Cui, Suping (Cui, Suping.) | Dai, Wenjing (Dai, Wenjing.) | Huang, Pingli (Huang, Pingli.) | Zhang, Boge (Zhang, Boge.) | Huang, Haibao (Huang, Haibao.)

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Scopus SCIE

摘要:

Nitrogen oxide emissions have attracted much attention due to their impact on the atmospheric environment and human health. Combined with NO removal in the cement production process, coal gasification slag was used to prepare denitrification materials to decompose NO in cement kilns without the addition of reducing agents. Denitrification materials were synthesized by a chemical precipitation method at different pH. The denitrification mechanism was proposed in this study. The results indicated that the denitrification material prepared at a pH of 7 exhibited the best denitrification performance. The NO decomposition rate first increased and then decreased below 400 degrees C, and then increased as the temperature increased, reaching over 97% above 700 degrees C. In the low-temperature range, Fe(II) was assumed to be active species, and the absorbed NO on the Fe(II) site obtained an electron, which promoted the decomposition of NO. In the high-temperature range, besides the active element Fe, the residual carbon in the coal gasification slag was prone to oxidation-reduction reactions, reducing nitric oxide to nitrogen. A new waste-to-value concept is introduced in this study, which promotes green technology for sustainable development.

关键词:

Residual carbon Coal gasification slag Cement kilns Denitrification performance Fe(II) ion

作者机构:

  • [ 1 ] [Gan, Yanling]Sun Yat sen Univ, Sch Environm Sci & Engn, 135 Xingang Xi Rd, Guangzhou 510275, Peoples R China
  • [ 2 ] [Gan, Yanling]Guangdong Hong Kong Macau Joint Lab Collaborat Inn, 855 Xingye Ave East, Hong Kong 511443, Guangdong, Peoples R China
  • [ 3 ] [Gan, Yanling]Beijing Univ Technol, Coll Mat Sci & Engn, 100 Pingleyuan, Beijing 100124, Peoples R China
  • [ 4 ] [Cui, Suping]Beijing Univ Technol, Coll Mat Sci & Engn, 100 Pingleyuan, Beijing 100124, Peoples R China
  • [ 5 ] [Dai, Wenjing]Sun Yat sen Univ, Sch Environm Sci & Engn, 135 Xingang Xi Rd, Guangzhou 510275, Peoples R China
  • [ 6 ] [Huang, Pingli]Sun Yat sen Univ, Sch Environm Sci & Engn, 135 Xingang Xi Rd, Guangzhou 510275, Peoples R China
  • [ 7 ] [Zhang, Boge]Sun Yat sen Univ, Sch Environm Sci & Engn, 135 Xingang Xi Rd, Guangzhou 510275, Peoples R China
  • [ 8 ] [Huang, Haibao]Sun Yat sen Univ, Sch Environm Sci & Engn, 135 Xingang Xi Rd, Guangzhou 510275, Peoples R China

通讯作者信息:

  • [Huang, Haibao]Sun Yat sen Univ, Sch Environm Sci & Engn, 135 Xingang Xi Rd, Guangzhou 510275, Peoples R China

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来源 :

JOURNAL OF ENVIRONMENTAL ENGINEERING

ISSN: 0733-9372

年份: 2024

期: 3

卷: 150

2 . 2 0 0

JCR@2022

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