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作者:

Liang Wenjun (Liang Wenjun.) (学者:梁文俊) | Guo Shuqing (Guo Shuqing.) | Ren Sida (Ren Sida.) | Li Qinglei (Li Qinglei.) | Li Jian (Li Jian.)

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SCIE

摘要:

The removal of low concentrations of toluene using non-thermal plasma (NTP) coupled with MnCe/La/cordierite honeycomb (CHB) catalysts had been investigated in this study. Mn/CHB, Mn-Ce/CHB, Mn-La/CHB catalysts were prepared for the experiment. The removal rate and removal amount of toluene, generation of O-3 and main aerosol by-products for different reactors had been investigated. The catalysts were characterized by BET, SEM, XRD and H-2-TPR. The results showed that rare earth catalysts could improve the removal efficiency of toluene and the degree of mineralization effectively. Mn-La/CHB catalyst had the better catalytic performance than Mn-Ce/CHB catalyst. The toluene removal rate and removal amount of Mn-La/CHB catalyst could be achieved at 76.31% and 159.0 mg/h, respectively, while the initial concentration of toluene being 600 mg/m(3), discharge voltage being 22kV and gas flow rate being 6 L/min. Moreover, H-2-TPR results showed that the low-temperature activity and capability of O-3 adsorption enhanced with the loading of rare earth catalysts. Catalysts were contributed to the decomposition of O-3.

关键词:

catalysis Mn-Ce/La/gamma-Al2O3 Non-thermal plasma ozone toluene

作者机构:

  • [ 1 ] [Liang Wenjun]Beijing Univ Technol, Key Lab Beijing Reg Air Pollut Control, Beijing 100124, Peoples R China
  • [ 2 ] [Guo Shuqing]Beijing Univ Technol, Key Lab Beijing Reg Air Pollut Control, Beijing 100124, Peoples R China
  • [ 3 ] [Ren Sida]Beijing Univ Technol, Key Lab Beijing Reg Air Pollut Control, Beijing 100124, Peoples R China
  • [ 4 ] [Li Qinglei]Beijing Univ Technol, Key Lab Beijing Reg Air Pollut Control, Beijing 100124, Peoples R China
  • [ 5 ] [Li Jian]Beijing Univ Technol, Key Lab Beijing Reg Air Pollut Control, Beijing 100124, Peoples R China

通讯作者信息:

  • 梁文俊

    [Liang Wenjun]Beijing Univ Technol, Key Lab Beijing Reg Air Pollut Control, Beijing 100124, Peoples R China

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来源 :

FRESENIUS ENVIRONMENTAL BULLETIN

ISSN: 1018-4619

年份: 2020

期: 1

卷: 29

页码: 473-480

ESI学科: ENVIRONMENT/ECOLOGY;

ESI高被引阀值:30

JCR分区:4

被引次数:

WoS核心集被引频次: 1

SCOPUS被引频次:

ESI高被引论文在榜: 0 展开所有

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