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作者:

Ji, Jie (Ji, Jie.) | Liu, Huijie (Liu, Huijie.) | Yao, Hui (Yao, Hui.) | You, Zhanping (You, Zhanping.)

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EI Scopus SCIE

摘要:

This study aims to investigate the effect of compatibilization methods on the compatibility between asphalt and direct coal liquefaction residue (DCLR) components to identify the key components in DCLR and asphalt that affect their compatibility. In this article, three types of compatibilizers, including benzyl alcohol (BA), dioctyl phthalate (DOP), and BA/DOP, were selected and acted on asphalt's components and DCLR's components, respectively. The molecular models of asphalt components, asphalt components with compatibilizers, DCLR components, and DCLR components with compatibilizers were established. The compatibility between DCLR and asphalt's four components, as well as between asphalt and DCLR's three components, were evaluated by solubility parameter difference (SPD) and interaction energy (IE). The compatibility between DCLR and asphalt was analyzed by Segregation test and Scanning Electron Microscope. Results indicate that the SPD and IE values between DCLR and asphalt components declined after adding compatibilizers, which implies that the repulsion decreased and the attraction increased between asphalt components and DCLR and the compatibility between asphalt components and DCLR improved. The IE values between DCLR components and asphalt increased after adding compatibilizers, which indicates that the compatibility was reduced between DCLR components and asphalt. The SPD values between DCLR components and asphalt increased after adding the BA/DOP. The SPD values between pre-asphaltene and asphalt decreased after adding the BA and DOP. The SPD value between asphaltene in DCLR and asphalt increased after adding the BA and decreased after adding the DOP. Moreover, the storage stability and homogeneity of DCLR-modified asphalt improved after adding compatibilizers, indicating that the compatibilizers enhanced compatibility between DCLR and asphalt. Finally, comparing the results of the tests, it could be found that compatibilizers preferentially acted on the asphalt components and mainly affected the aromatics in asphalt, thereby improving the compatibility between asphalt and DCLR. The effect of BA/DOP on improving the compatibility between asphalt and DCLR was better than that of BA and DOP.

关键词:

Molecular dynamics Direct coal liquefaction residue (DCLR) Compatibility DCLR-modified asphalt Compatibilizer

作者机构:

  • [ 1 ] [Ji, Jie]Beijing Univ Civil Engn & Architecture, Sch Civil Engn & Transportat, Beijing 100044, Peoples R China
  • [ 2 ] [Liu, Huijie]Beijing Univ Technol, Coll Metropolitan Transportat, Beijing Key Lab Traff Engn, 100 Pingleyuan, Beijing 100124, Peoples R China
  • [ 3 ] [Yao, Hui]Beijing Univ Technol, Coll Metropolitan Transportat, Beijing Key Lab Traff Engn, 100 Pingleyuan, Beijing 100124, Peoples R China
  • [ 4 ] [You, Zhanping]Michigan Technol Univ, Dept Civil & Environm Engn, 1400 Townsend Dr, Houghton, MI 49931 USA

通讯作者信息:

  • [Yao, Hui]Beijing Univ Technol, Coll Metropolitan Transportat, Beijing Key Lab Traff Engn, 100 Pingleyuan, Beijing 100124, Peoples R China;;

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来源 :

CONSTRUCTION AND BUILDING MATERIALS

ISSN: 0950-0618

年份: 2024

卷: 431

7 . 4 0 0

JCR@2022

被引次数:

WoS核心集被引频次: 3

SCOPUS被引频次: 4

ESI高被引论文在榜: 0 展开所有

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中文被引频次:

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