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作者:

Lu, Mengzhe (Lu, Mengzhe.) | Chang, Haiqing (Chang, Haiqing.) | Yan, Zhongsen (Yan, Zhongsen.) | Qu, Fangshu (Qu, Fangshu.) | Zhou, Zhiwei (Zhou, Zhiwei.) | Liang, Ying (Liang, Ying.) | Zhao, Huaxin (Zhao, Huaxin.) | Liu, Naiming (Liu, Naiming.) | Ren, Li (Ren, Li.) | Liang, Heng (Liang, Heng.)

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EI Scopus SCIE

摘要:

Shale gas is abundant worldwide and has a smaller carbon footprint than conventional coal. However, exploitation of shale gas produces a large amount of hydraulic fracturing wastewater, which hurts the ecological environment. Effective treatment of shale gas produced water (SGPW) is a great challenge and membrane distillation (MD) which is not restricted by salinity is a hot topic in dealing with this wastewater. This paper focused on the influence of feed water quality on performance of direct contact MD by adjusting pH and pretreating. By analyzing MD permeate, controlling the feed water non-alkalinity facilitated MD treatment of SGPW and acidic condition greatly hindered the cross -membrane mass transfer of ammonia nitrogen. Among the traditional pretreatment methods, aluminum coagulant removed 99% of turbidity and exhibited the best superiority in mitigating membrane fouling, whose final flux was 2.2 times the raw SGPW. Dual coagulation and zeolite adsorption reduced ammonia nitrogen by about 50 % and 95 %, whose final permeate conductivities were about 65 % and 62 % of the untreated, respectively. Analyses of attenuated total reflection fourier transform infrared and scanning electron microscope equipped with an energy dispersive spectroscopy confirmed the reduction in membrane fouling after pretreatment of feed water. This study provides guidance for treatment of SGPW using MD.

关键词:

Membrane fouling Shale gas produced water (SGPW) Ammonia transfer Membrane distillation (MD) Feed water quality

作者机构:

  • [ 1 ] [Lu, Mengzhe]Sichuan Univ, Coll Architecture & Environm, MOE Key Lab Deep Earth Sci & Engn, Chengdu 610207, Peoples R China
  • [ 2 ] [Chang, Haiqing]Sichuan Univ, Coll Architecture & Environm, MOE Key Lab Deep Earth Sci & Engn, Chengdu 610207, Peoples R China
  • [ 3 ] [Liang, Ying]Sichuan Univ, Coll Architecture & Environm, MOE Key Lab Deep Earth Sci & Engn, Chengdu 610207, Peoples R China
  • [ 4 ] [Zhao, Huaxin]Sichuan Univ, Coll Architecture & Environm, MOE Key Lab Deep Earth Sci & Engn, Chengdu 610207, Peoples R China
  • [ 5 ] [Liu, Naiming]Sichuan Univ, Coll Architecture & Environm, MOE Key Lab Deep Earth Sci & Engn, Chengdu 610207, Peoples R China
  • [ 6 ] [Ren, Li]Sichuan Univ, Coll Architecture & Environm, MOE Key Lab Deep Earth Sci & Engn, Chengdu 610207, Peoples R China
  • [ 7 ] [Yan, Zhongsen]Fuzhou Univ, Coll Civil Engn, Fuzhou 350116, Fujian, Peoples R China
  • [ 8 ] [Qu, Fangshu]Guangzhou Univ, Sch Civil Engn, Guangzhou 510006, Peoples R China
  • [ 9 ] [Zhou, Zhiwei]Beijing Univ Technol, Coll Architecture & Civil Engn, Fac Urban Construct, Beijing 100124, Peoples R China
  • [ 10 ] [Liang, Heng]Harbin Inst Technol, State Key Lab Urban Water Resource & Environm SKLU, Harbin 150090, Peoples R China

通讯作者信息:

  • [Chang, Haiqing]Sichuan Univ, Coll Architecture & Environm, MOE Key Lab Deep Earth Sci & Engn, Chengdu 610207, Peoples R China;;

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来源 :

SEPARATION AND PURIFICATION TECHNOLOGY

ISSN: 1383-5866

年份: 2024

卷: 341

8 . 6 0 0

JCR@2022

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SCOPUS被引频次: 13

ESI高被引论文在榜: 0 展开所有

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