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作者:

Zhang, Wen-Hai (Zhang, Wen-Hai.) | Ren, Yun-Han (Ren, Yun-Han.) | Yin, Ming-Jie (Yin, Ming-Jie.) | Liu, Zhi-Jie (Liu, Zhi-Jie.) | Gao, Haiqi (Gao, Haiqi.) | Wang, Shuang-Shuang (Wang, Shuang-Shuang.) | Wang, Zhen-Yuan (Wang, Zhen-Yuan.) | An, Quan-Fu (An, Quan-Fu.) (学者:安全福) | Meng, Hong (Meng, Hong.)

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EI Scopus SCIE

摘要:

Graphene oxide (GO) is regarded as a promising next-generation high-performance separation membrane material. However, the flexiblility of single-layer GO nanosheets usually results in membrane with poor stability under practical conditions. In this study, we present a facile strategy to rapidly convert single-layer nanosheet GO membranes into supra-nanosheet GO (sGO) membranes with a loose rigid structure by a confined gelling and crosslinking process. The optimized sGO membrane exhibits remarkable water permeance and retention capability. With additional tailor-made nanopores, the water permeance of the sGO membrane could reach 52.0 LMH/bar, representing 10-fold increase compared to pristine GO membrane. Furtheermore, this membrane demonstrates excellent pressure stability and unique elasticity, enhancing its lorg-term operational reliability and reversible recovery. Hence, this innovative strategy provides a platform for the facily construction of highly stable 2D membranes with enhanced water transport channels.

关键词:

Loose nanofiltration Supra-GO (sGO) GO membrane Antibiotic desalination Crosslinking

作者机构:

  • [ 1 ] [Zhang, Wen-Hai]Xinjiang Univ, Coll Chem, State Key Lab Chem & Utilizat Carbon Based Energy, Urumqi 830017, Xinjiang, Peoples R China
  • [ 2 ] [Gao, Haiqi]Xinjiang Univ, Coll Chem, State Key Lab Chem & Utilizat Carbon Based Energy, Urumqi 830017, Xinjiang, Peoples R China
  • [ 3 ] [Meng, Hong]Xinjiang Univ, Coll Chem, State Key Lab Chem & Utilizat Carbon Based Energy, Urumqi 830017, Xinjiang, Peoples R China
  • [ 4 ] [Ren, Yun-Han]Beijing Univ Technol, Coll Mat Sci & Engn, Dept Chem Engn, Beijing Key Lab Green Catalysis & Separat, Beijing 100124, Peoples R China
  • [ 5 ] [Yin, Ming-Jie]Beijing Univ Technol, Coll Mat Sci & Engn, Dept Chem Engn, Beijing Key Lab Green Catalysis & Separat, Beijing 100124, Peoples R China
  • [ 6 ] [Liu, Zhi-Jie]Beijing Univ Technol, Coll Mat Sci & Engn, Dept Chem Engn, Beijing Key Lab Green Catalysis & Separat, Beijing 100124, Peoples R China
  • [ 7 ] [An, Quan-Fu]Beijing Univ Technol, Coll Mat Sci & Engn, Dept Chem Engn, Beijing Key Lab Green Catalysis & Separat, Beijing 100124, Peoples R China
  • [ 8 ] [Wang, Shuang-Shuang]Beijing Univ Technol, Large Scale Instruments & Equipments Sharing Plate, Beijing 100124, Peoples R China
  • [ 9 ] [Wang, Zhen-Yuan]Univ Suzhou, NJTECH, Future Membrane Technol Innovat Ctr, Suzhou, Peoples R China

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来源 :

JOURNAL OF MEMBRANE SCIENCE

ISSN: 0376-7388

年份: 2024

卷: 711

9 . 5 0 0

JCR@2022

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SCOPUS被引频次: 5

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