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作者:

Gao, Jing-Feng (Gao, Jing-Feng.) (学者:高景峰) | Wu, Zhi-Long (Wu, Zhi-Long.) | Duan, Wan-Jun (Duan, Wan-Jun.) | Zhang, Wen-Zhi (Zhang, Wen-Zhi.)

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摘要:

Triclosan (TCS), an antimicrobial agent added in many pharmaceutical and personal care products, can cause some environmental problems due to its bioaccumulation, toxicity and potential antibiotic cross-resistance. In this study, Ginkgo biloba L. leaf extract was used as the green stabilizing agent to synthesize Fe/Co bimetallic nanoparticles (G-Fe/Co NPs), which were applied to remove TCS from aqueous solution. G-Fe/Co NPs were characterized by TEM, EDS, SEM, BET, FTIR, XRD and XPS. G. biloba L. leaf extract improved the dispersion and reduced the passivation of NPs. The TCS removal efficiency followed the order of G-Fe/Co NPs > G-Fe NPs > Co NPs > Fe/Co NPs > Fe NPs. G-Fe/Co NPs can be reused at least eight times. The Co leaching under different initial pH values was negligible. The factors affecting the TCS removal were investigated. The results indicated that the removal of TCS followed pseudo-second-order kinetics, and the removal rate constant decreased with increasing the initial pH value and the initial TCS concentration, and decreasing the Co loading of G-Fe/Co NPs and NPs dosage. The mass balance of TCS removal by G-Fe/Co NPs indicated that adsorption was dominant process and TCS degradation was an accumulative process. (C) 2019 Elsevier B.V. All rights reserved.

关键词:

Adsorption Ginkgo biloba L. Triclosan Fe/Co bimetallic Degradation

作者机构:

  • [ 1 ] [Gao, Jing-Feng]Beijing Univ Technol, Natl Engn Lab Adv Municipal Wastewater Treatment, Beijing 100124, Peoples R China
  • [ 2 ] [Wu, Zhi-Long]Beijing Univ Technol, Natl Engn Lab Adv Municipal Wastewater Treatment, Beijing 100124, Peoples R China
  • [ 3 ] [Duan, Wan-Jun]Beijing Univ Technol, Natl Engn Lab Adv Municipal Wastewater Treatment, Beijing 100124, Peoples R China
  • [ 4 ] [Zhang, Wen-Zhi]Beijing Univ Technol, Natl Engn Lab Adv Municipal Wastewater Treatment, Beijing 100124, Peoples R China

通讯作者信息:

  • 高景峰

    [Gao, Jing-Feng]Beijing Univ Technol, Natl Engn Lab Adv Municipal Wastewater Treatment, Beijing 100124, Peoples R China

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来源 :

SCIENCE OF THE TOTAL ENVIRONMENT

ISSN: 0048-9697

年份: 2019

卷: 662

页码: 978-989

9 . 8 0 0

JCR@2022

ESI学科: ENVIRONMENT/ECOLOGY;

ESI高被引阀值:167

JCR分区:1

被引次数:

WoS核心集被引频次: 40

SCOPUS被引频次: 42

ESI高被引论文在榜: 0 展开所有

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