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作者:

Wang, Yifei (Wang, Yifei.) | Yang, Qing (Yang, Qing.) | Huang, Haiou (Huang, Haiou.)

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摘要:

In this study, carbon nanotube (CNT) and reduced graphene oxide (rGO) were studied for their potentials as novel adsorbents for trace concentrations of phosphorus and aluminum in water and wastewater. Static adsorption results demonstrated that CNT and rGO employed in this study removed up to 65.6% of total dissolved Al and 98.9% of P from a natural surface water and a secondary wastewater effluent. Hydrogen-bonding interactions between CNT/rGO and oxyanions were hypothesized to contribute to the adsorption process. Accordingly, acetaminophen (AAP), a pharmaceutical compound known to form hydrogen bonding with CNT, was spiked into the real water as a competitor for P and Al adsorption. Subsequent sorption results showed that the presence of AAP reduced Al and P adsorption by CNT and rGO by 9.3%-18.4% and 11.2%-18.2%, respectively. These results suggest that hydrogen bonding interactions with CNT/rGO influenced the adsorption of P and Al species. In addition, pH effect investigation on Al/P removal further verified the above opinion. Overall, this study provided important evidence and insights into CNT/rGO adsorption of P and Al species from water and wastewater, which expanded our understanding on the ability of carbonaceous nanomaterials for advanced water and wastewater treatment. (c) 2019 Elsevier B.V. All rights reserved.

关键词:

Acetaminophen Adsorption Hydrogen bonding Nanomaterials Trace phosphate and aluminum

作者机构:

  • [ 1 ] [Wang, Yifei]Beijing Univ Technol, Natl Engn Lab Adv Municipal Wastewater Treatment, Key Lab Beijing Water Qual Sci & Water Environm R, Beijing 100124, Peoples R China
  • [ 2 ] [Wang, Yifei]Beijing Normal Univ, Sch Environm, State Key Joint Lab Environm Simulat & Pollut Con, 19 Xinjiekouwai St, Beijing 100875, Peoples R China
  • [ 3 ] [Yang, Qing]Beijing Normal Univ, Sch Environm, State Key Joint Lab Environm Simulat & Pollut Con, 19 Xinjiekouwai St, Beijing 100875, Peoples R China
  • [ 4 ] [Huang, Haiou]Beijing Normal Univ, Sch Environm, State Key Joint Lab Environm Simulat & Pollut Con, 19 Xinjiekouwai St, Beijing 100875, Peoples R China
  • [ 5 ] [Huang, Haiou]Johns Hopkins Univ, Bloomberg Sch Publ Hlth, Dept Environm Hlth & Engn, 615 North Wolfe St, Baltimore, MD 21205 USA

通讯作者信息:

  • [Huang, Haiou]Beijing Normal Univ, Sch Environm, State Key Joint Lab Environm Simulat & Pollut Con, 19 Xinjiekouwai St, Beijing 100875, Peoples R China

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来源 :

SCIENCE OF THE TOTAL ENVIRONMENT

ISSN: 0048-9697

年份: 2019

卷: 662

页码: 1003-1011

9 . 8 0 0

JCR@2022

ESI学科: ENVIRONMENT/ECOLOGY;

ESI高被引阀值:57

JCR分区:1

被引次数:

WoS核心集被引频次: 23

SCOPUS被引频次: 28

ESI高被引论文在榜: 0 展开所有

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