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作者:

Liu, Haijiao (Liu, Haijiao.) | Yan, Yan (Yan, Yan.) | Chang, Hong (Chang, Hong.) | Chen, Hongyun (Chen, Hongyun.) | Liang, Lianji (Liang, Lianji.) | Liu, Xingxing (Liu, Xingxing.) | Qiang, Xiaoke (Qiang, Xiaoke.) | Sun, Youbin (Sun, Youbin.)

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Scopus SCIE

摘要:

The characteristics of urban dust aerosols and the contributions of their natural and anthropogenic sources are of scientific interest as well as being of substantial sociopolitical and economic concern. Here we present a comprehensive study of dust flux, magnetic parameters, magnetic particulate morphology, and elemental compositions of atmospheric dustfall originating from natural dust sources in East Asia and local anthropogenic sources in Xi'an, China. The results reveal a significant inverse relationship between seasonal variations of dust flux and magnetic susceptibility (chi). By comparing dust flux and chi records, the relative contributions of dust from local anthropogenic sources are estimated. Analyses using scanning electron microscopy (SEM) combined with energy dispersive spectroscopy (EDS) indicate that magnetic particulate from different sources has distinct morphological and elemental characteristics. Detrital magnetic particles originating from natural sources are characterized by relatively smooth surfaces with Fe and O as the major elements and a minor contribution from Ti. The anthropogenic particles have angular, spherical, aggregate, and porous shapes with distinctive contributions from marker elements, including S, Cr, Cu, Zn, Ni, Mn, and Ca. Our results demonstrate that this multidisciplinary approach is effective in distinguishing dust particles derived from distant natural sources and local anthropogenic sources and for the quantitative assessment of contributions from the two end-members.

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作者机构:

  • [ 1 ] [Liu, Haijiao]Chinese Acad Sci, Inst Earth Environm, State Key Lab Loess & Quaternary Geol, Xian 710061, Shaanxi, Peoples R China
  • [ 2 ] [Chang, Hong]Chinese Acad Sci, Inst Earth Environm, State Key Lab Loess & Quaternary Geol, Xian 710061, Shaanxi, Peoples R China
  • [ 3 ] [Liu, Xingxing]Chinese Acad Sci, Inst Earth Environm, State Key Lab Loess & Quaternary Geol, Xian 710061, Shaanxi, Peoples R China
  • [ 4 ] [Qiang, Xiaoke]Chinese Acad Sci, Inst Earth Environm, State Key Lab Loess & Quaternary Geol, Xian 710061, Shaanxi, Peoples R China
  • [ 5 ] [Sun, Youbin]Chinese Acad Sci, Inst Earth Environm, State Key Lab Loess & Quaternary Geol, Xian 710061, Shaanxi, Peoples R China
  • [ 6 ] [Liu, Haijiao]Univ Chinese Acad Sci, Coll Earth Sci, Beijing 100049, Peoples R China
  • [ 7 ] [Yan, Yan]Chinese Acad Sci, Guangzhou Inst Geochem, Key Lab Ocean & Marginal Sea Geol, Guangzhou 510640, Guangdong, Peoples R China
  • [ 8 ] [Chang, Hong]Chinese Acad Sci, CAS Ctr Excellence Quaternary Sci & Global Change, Xian 710061, Shaanxi, Peoples R China
  • [ 9 ] [Liu, Xingxing]Chinese Acad Sci, CAS Ctr Excellence Quaternary Sci & Global Change, Xian 710061, Shaanxi, Peoples R China
  • [ 10 ] [Qiang, Xiaoke]Chinese Acad Sci, CAS Ctr Excellence Quaternary Sci & Global Change, Xian 710061, Shaanxi, Peoples R China
  • [ 11 ] [Sun, Youbin]Chinese Acad Sci, CAS Ctr Excellence Quaternary Sci & Global Change, Xian 710061, Shaanxi, Peoples R China
  • [ 12 ] [Chen, Hongyun]Chinese Acad Geol Sci, Res Ctr Loess & Global Changes, Inst Hydrogeol & Environm Geol, Shijiazhuang 050803, Hebei, Peoples R China
  • [ 13 ] [Liang, Lianji]Beijing Univ Technol, Coll Architecture & Civil Engn, Beijing 100124, Peoples R China
  • [ 14 ] [Sun, Youbin]Xi An Jiao Tong Univ, Inst Global Environm Change, Xian 710049, Shaanxi, Peoples R China

通讯作者信息:

  • [Sun, Youbin]Chinese Acad Sci, Inst Earth Environm, State Key Lab Loess & Quaternary Geol, Xian 710061, Shaanxi, Peoples R China;;[Sun, Youbin]Chinese Acad Sci, CAS Ctr Excellence Quaternary Sci & Global Change, Xian 710061, Shaanxi, Peoples R China;;[Sun, Youbin]Xi An Jiao Tong Univ, Inst Global Environm Change, Xian 710049, Shaanxi, Peoples R China

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来源 :

ATMOSPHERIC CHEMISTRY AND PHYSICS

ISSN: 1680-7316

年份: 2019

期: 2

卷: 19

页码: 731-745

6 . 3 0 0

JCR@2022

ESI学科: GEOSCIENCES;

ESI高被引阀值:123

JCR分区:1

被引次数:

WoS核心集被引频次: 33

SCOPUS被引频次: 34

ESI高被引论文在榜: 0 展开所有

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