• 综合
  • 标题
  • 关键词
  • 摘要
  • 学者
  • 期刊-刊名
  • 期刊-ISSN
  • 会议名称
搜索

作者:

Liang, Q. (Liang, Q..) | Liang, W. (Liang, W..) | Fan, X. (Fan, X..) | Song, L. (Song, L..) | Li, J. (Li, J..) (学者:李坚) | He, H. (He, H..) (学者:何洪)

收录:

Scopus PKU CSCD

摘要:

The effects of V2O5 loading, the volume fractions of O2, NO, SO2 and H2O, n(NH3)/n(NO), gas hourly space velocity and online heat regeneration on NO conversion of V2O5-WO3/TiO2 catalyst prepared by impregnation method were investigated. Combined with the experimental results, 3% V2O5 was selected as the optimal loading, and NO conversion of 3% V2O5-WO3/TiO2 catalyst was 93.7% at 160 ℃. The selectivity of N2 was more than 98% and SO2 oxidation was less than 1% in the range of 110-320 ℃. NO conversion of catalyst increased with the increase of the volume fraction of O2, and decreased with the increase of the volume fraction of NO, however, the NOx removal amount gradually increased. When n(NH3)/n(NO)≤1, the optimal activity of catalyst equalled the respective n(NH3)/n(NO), and when n(NH3)/n(NO)>1, the activity was barely improved. With the increase of the space velocity, the high activity temperature range of the catalyst was narrowed, and the activity decreased in varying degrees. The characterization results show that the morphology of catalyst is blurred and the surface covered with irregular flocs, specific surface area and pore volume decrease in different degrees, and tiny pores are preferred to be blocked after selective catalytic reduction (SCR) reaction containing SO2 and H2O. The contents of V2O5 are reduced 0.98% and WO3 reduced 1.6%, the side reaction products include NH4 + and SO4 2-. During the process of online heat regeneration, catalyst delayed the decomposition of ammonium sulfate, which caused the catalyst's resistance to poisoning to be worse and the activity was difficult to be recover. © 2019, Editorial Department of Journal of Beijing University of Technology. All right reserved.

关键词:

Different flue gas conditions; Low temperature SCR; Non electric power industry; Online heat regeneration; V2O5-WO3/TiO2

作者机构:

  • [ 1 ] [Liang, Q.]Key Laboratory of Beijing on Regional Air Pollution Control, Beijing university of Technology, Beijing, 100124, China
  • [ 2 ] [Liang, Q.]Beijing Key Laboratory for Green Catalysis and Separation, Beijing university of Technology, Beijing, 100124, China
  • [ 3 ] [Liang, Q.]Beijing Municipal Institute of Labor Protection, Beijing, 100054, China
  • [ 4 ] [Liang, W.]Key Laboratory of Beijing on Regional Air Pollution Control, Beijing university of Technology, Beijing, 100124, China
  • [ 5 ] [Liang, W.]Beijing Key Laboratory for Green Catalysis and Separation, Beijing university of Technology, Beijing, 100124, China
  • [ 6 ] [Fan, X.]Key Laboratory of Beijing on Regional Air Pollution Control, Beijing university of Technology, Beijing, 100124, China
  • [ 7 ] [Fan, X.]Beijing Key Laboratory for Green Catalysis and Separation, Beijing university of Technology, Beijing, 100124, China
  • [ 8 ] [Song, L.]Key Laboratory of Beijing on Regional Air Pollution Control, Beijing university of Technology, Beijing, 100124, China
  • [ 9 ] [Song, L.]Beijing Key Laboratory for Green Catalysis and Separation, Beijing university of Technology, Beijing, 100124, China
  • [ 10 ] [Li, J.]Key Laboratory of Beijing on Regional Air Pollution Control, Beijing university of Technology, Beijing, 100124, China
  • [ 11 ] [Li, J.]Beijing Key Laboratory for Green Catalysis and Separation, Beijing university of Technology, Beijing, 100124, China
  • [ 12 ] [He, H.]Key Laboratory of Beijing on Regional Air Pollution Control, Beijing university of Technology, Beijing, 100124, China
  • [ 13 ] [He, H.]Beijing Key Laboratory for Green Catalysis and Separation, Beijing university of Technology, Beijing, 100124, China

通讯作者信息:

  • 李坚

    [Li, J.]Key Laboratory of Beijing on Regional Air Pollution Control, Beijing university of TechnologyChina

电子邮件地址:

查看成果更多字段

相关关键词:

相关文章:

来源 :

Journal of Beijing University of Technology

ISSN: 0254-0037

年份: 2019

期: 7

卷: 45

页码: 699-709

被引次数:

WoS核心集被引频次: 0

SCOPUS被引频次: 1

ESI高被引论文在榜: 0 展开所有

万方被引频次:

中文被引频次:

近30日浏览量: 0

在线人数/总访问数:659/3900405
地址:北京工业大学图书馆(北京市朝阳区平乐园100号 邮编:100124) 联系我们:010-67392185
版权所有:北京工业大学图书馆 站点建设与维护:北京爱琴海乐之技术有限公司