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Author:

Shi, Xiao-Lei (Shi, Xiao-Lei.) | Zheng, Kun (Zheng, Kun.) (Scholars:郑坤) | Liu, Wei-Di (Liu, Wei-Di.) | Wang, Yuan (Wang, Yuan.) | Yang, Yu-Zhe (Yang, Yu-Zhe.) | Chen, Zhi-Gang (Chen, Zhi-Gang.) | Zou, Jin (Zou, Jin.)

Indexed by:

EI Scopus SCIE

Abstract:

In this study, a record high figure of merit (ZT) of approximate to 1.1 at 773 K is reported in n-type highly distorted Sb-doped SnSe microplates via a facile solvothermal method. The pellets sintered from the Sb-doped SnSe microplates show a high power factor of approximate to 2.4 mu W cm(-1) K-2 and an ultralow thermal conductivity of approximate to 0.17 W m(-1) K-1 at 773 K, leading a record high ZT. Such a high power factor is attributed to a high electron concentration of 3.94 x 10(19) cm(-3) via Sb-enabled electron doping, and the ultralow thermal conductivity derives from the enhanced phonon scattering at intensive crystal defects, including severe lattice distortions, dislocations, and lattice bent, observed by detailed structural characterizations. This study fills in the gaps of fundamental doping mechanisms of Sb in SnSe system, and provides a new perspective to achieve high thermoelectric performance in n-type polycrystalline SnSe.

Keyword:

n-type doping thermoelectric materials solvothermal synthesis tin selenide thermal conductivity

Author Community:

  • [ 1 ] [Shi, Xiao-Lei]Univ Queensland, Mat Engn, Brisbane, Qld 4072, Australia
  • [ 2 ] [Liu, Wei-Di]Univ Queensland, Mat Engn, Brisbane, Qld 4072, Australia
  • [ 3 ] [Yang, Yu-Zhe]Univ Queensland, Mat Engn, Brisbane, Qld 4072, Australia
  • [ 4 ] [Chen, Zhi-Gang]Univ Queensland, Mat Engn, Brisbane, Qld 4072, Australia
  • [ 5 ] [Zou, Jin]Univ Queensland, Mat Engn, Brisbane, Qld 4072, Australia
  • [ 6 ] [Zheng, Kun]Beijing Univ Technol, Inst Microstruct & Properties Adv Mat, Beijing 100022, Peoples R China
  • [ 7 ] [Wang, Yuan]Univ Southern Queensland, Ctr Future Mat, Springfield, Qld 4300, Australia
  • [ 8 ] [Chen, Zhi-Gang]Univ Southern Queensland, Ctr Future Mat, Springfield, Qld 4300, Australia
  • [ 9 ] [Zou, Jin]Univ Queensland, Ctr Microscopy & Microanal, Brisbane, Qld 4072, Australia

Reprint Author's Address:

  • [Chen, Zhi-Gang]Univ Queensland, Mat Engn, Brisbane, Qld 4072, Australia;;[Zou, Jin]Univ Queensland, Mat Engn, Brisbane, Qld 4072, Australia;;[Chen, Zhi-Gang]Univ Southern Queensland, Ctr Future Mat, Springfield, Qld 4300, Australia;;[Zou, Jin]Univ Queensland, Ctr Microscopy & Microanal, Brisbane, Qld 4072, Australia

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Source :

ADVANCED ENERGY MATERIALS

ISSN: 1614-6832

Year: 2018

Issue: 21

Volume: 8

2 7 . 8 0 0

JCR@2022

ESI Discipline: MATERIALS SCIENCE;

ESI HC Threshold:260

JCR Journal Grade:1

Cited Count:

WoS CC Cited Count: 135

SCOPUS Cited Count: 134

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 2

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