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作者:

Yang, Xiaowen (Yang, Xiaowen.) | Cheng, Shuiyuan (Cheng, Shuiyuan.) (学者:程水源) | Wang, Gang (Wang, Gang.) | Xu, Ran (Xu, Ran.) | Wang, Xiaoqi (Wang, Xiaoqi.) | Zhang, Hanyu (Zhang, Hanyu.) | Chen, Guolei (Chen, Guolei.)

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摘要:

In this study, the measurement of volatile organic compounds (VOCs) was conducted at Beijing Capital International Airport (ZBAA) and a background reference site in four seasons of 2015. Total concentrations of VOCs were 72.6 +/- 9.7, 65.5 +/- 8.7, 95.8 +/- 11.0, and 79.2 +/- 10.8 mu g/m(3) in winter, spring, summer, and autumn, respectively. The most abundant specie was toluene (10.1%-17.4%), followed by benzene, ethane, isopentane, ethane, acetylene, and n-butane. Seasonal variations of VOCs were analyzed, and it was found that the highest concentration occurring in summer, while the lowest in spring. For the diurnal variation, the concentration of V005 in the daytime (9:00-15:00) was less than that at night (15:00-21:00) obviously. Ozone Formation Potential (OFP) was calculated by using Maximum Incremental Reactivity (MIR) method. The greatest contribution to OFP from alkenes and aromatics, which accounted for 27.3%-51.2% and 36.6%-58.6% of the total OFP. The WRF-CMAQ model was used to simulate the impact of airport emissions on the surrounding area. The results indicated that the maximum impact of VOCs emissions and all sources emissions at the airport on O-3 was 0.035 and 23.8 mu g/m(3), respectively. Meanwhile, within 1 km from the airport, the concentration of O-3 around the airport was greatly affected by airport emitted. (C) 2018 Published by Elsevier Ltd.

关键词:

Beijing capital international airport Ozone formation potential Temporal variation Volatile organic compounds (VOCs) WRF-CMAQ

作者机构:

  • [ 1 ] [Yang, Xiaowen]Beijing Univ Technol, Key Lab Beijing Reg Air Pollut Control, Beijing 100124, Peoples R China
  • [ 2 ] [Cheng, Shuiyuan]Beijing Univ Technol, Key Lab Beijing Reg Air Pollut Control, Beijing 100124, Peoples R China
  • [ 3 ] [Wang, Gang]Beijing Univ Technol, Key Lab Beijing Reg Air Pollut Control, Beijing 100124, Peoples R China
  • [ 4 ] [Wang, Xiaoqi]Beijing Univ Technol, Key Lab Beijing Reg Air Pollut Control, Beijing 100124, Peoples R China
  • [ 5 ] [Zhang, Hanyu]Beijing Univ Technol, Key Lab Beijing Reg Air Pollut Control, Beijing 100124, Peoples R China
  • [ 6 ] [Chen, Guolei]Beijing Univ Technol, Key Lab Beijing Reg Air Pollut Control, Beijing 100124, Peoples R China
  • [ 7 ] [Cheng, Shuiyuan]Collaborat Innovat Ctr Elect Vehicles Beijing, Beijing 100081, Peoples R China
  • [ 8 ] [Xu, Ran]Natl Meteorol Ctr CMA, Beijing 100081, Peoples R China

通讯作者信息:

  • 程水源

    [Cheng, Shuiyuan]Beijing Univ Technol, Key Lab Beijing Reg Air Pollut Control, Beijing 100124, Peoples R China

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来源 :

ENVIRONMENTAL POLLUTION

ISSN: 0269-7491

年份: 2018

卷: 238

页码: 491-499

8 . 9 0 0

JCR@2022

ESI学科: ENVIRONMENT/ECOLOGY;

ESI高被引阀值:89

JCR分区:1

被引次数:

WoS核心集被引频次: 18

SCOPUS被引频次: 21

ESI高被引论文在榜: 0 展开所有

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